Gradient Electronic Landscapes in van der Waals Heterostructures

Two-dimensional (2D) materials, such as graphene and hexagonal boron nitride (hBN), provide a versatile platform for quantum electronics. Experiments generally require encapsulation of graphene within hBN flakes, forming a protective van der Waals (vdW) heterostructure that preserves the delicate properties of the embedded crystal. To produce functional devices, heterostructures are typically shaped by electron beam lithography and etching, which have driven progress in 2D materials research. However, patterns are primarily restricted to in-plane geometries such as boxes, holes, and stripes, limiting opportunities for advanced architectures. Here, we use thermal scanning-probe lithography to produce smooth topographic landscapes in vdW heterostructures by patterning the thickness of the top hBN flake with nanometer precision. We electrically gate a sinusoidal topography to impose a periodic electric-field gradient on the graphene layer to spatially modulate charge-carrier density. We observe signatures of the landscape in transport measurements─resistance-peak spreading and commensurability oscillations─establishing this approach for tailoring mathematically precise potentials in quantum electronics.

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Publication Details

Journal
Nano Letters
Published
2025-12-03
DOI
https://doi.org/10.1021/acs.nanolett.5c05437
Primary Topic
Graphene research and applications
Type
article
Field-Weighted Citation Impact
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article

Gradient Electronic Landscapes in van der Waals Heterostructures

Giulia Meucci, Peter Bøggild, Timothy J. Booth, Nolan Lassaline et al.
Nano Letters
Graphene research and applications
article

Gradient Electronic Landscapes in van der Waals Heterostructures

Giulia Meucci, Peter Bøggild, Timothy J. Booth, Nolan Lassaline, Thomas Sand Jespersen, Tuan Khanh Chau, Damon J. Carrad, Camilla Sørensen, Magnus V. Nielsen, Sander J. Linde, Kian Latifi Yaghin
article en

Abstract

Two-dimensional (2D) materials, such as graphene and hexagonal boron nitride (hBN), provide a versatile platform for quantum electronics. Experiments generally require encapsulation of graphene within hBN flakes, forming a protective van der Waals (vdW) heterostructure that preserves the delicate properties of the embedded crystal. To produce functional devices, heterostructures are typically shaped by electron beam lithography and etching, which have driven progress in 2D materials research. However, patterns are primarily restricted to in-plane geometries such as boxes, holes, and stripes, limiting opportunities for advanced architectures. Here, we use thermal scanning-probe lithography to produce smooth topographic landscapes in vdW heterostructures by patterning the thickness of the top hBN flake with nanometer precision. We electrically gate a sinusoidal topography to impose a periodic electric-field gradient on the graphene layer to spatially modulate charge-carrier density. We observe signatures of the landscape in transport measurements─resistance-peak spreading and commensurability oscillations─establishing this approach for tailoring mathematically precise potentials in quantum electronics.

Nano LettersVol. 25(50)
Technical University of Denmark (DK)
Openalex Percentile: Top 69%
Graphene research and applications
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