Molten Embedded Writing of End-Use Thermoplastics for Engineering Applications

Fused filament fabrication has been applied to manufacture complex thermoplastic structures. However, due to the poor mechanical strength, the printed structures are typically used for prototyping purposes rather than end-use functional parts. Inspired by embedded ink writing, which produces three-dimensional architectures with enhanced mechanical properties, a molten embedded writing (MEW) method is developed in this work to print thermoplastic polymer filaments within a high-temperature support bath. The support bath is composed of organomodified montmorillonite particles and high-smoking-point sunflower oil, which offers a desired thermal environment to promote interfilament fusion, thereby enhancing the mechanical strength of as-printed structures. To demonstrate the broad and reliable application of MEW, three representative end-use parts, including orbital implants from polycaprolactone, spigots from polylactic acid for a lab-scale hydrocyclone, and sensors from thermal polyurethane, are successfully printed for repairing an orbital bone fracture, enhancing mineral particle separation, and detecting strain and force for a robotic hand, respectively.

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Journal
ACS Applied Materials & Interfaces
Published
2025-12-01
DOI
https://doi.org/10.1021/acsami.5c16456
Primary Topic
Additive Manufacturing and 3D Printing Technologies
Type
article
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article

Molten Embedded Writing of End-Use Thermoplastics for Engineering Applications

Dale K. Hensley, Erick R. Bandala, Katy Juárez, Aidan Shackleford et al.
ACS Applied Materials & Interfaces
Additive Manufacturing and 3D Printing Technologies
article

Molten Embedded Writing of End-Use Thermoplastics for Engineering Applications

Dale K. Hensley, Erick R. Bandala, Katy Juárez, Aidan Shackleford, Kellen Mitchell, Guangrui Chai, Ji Su, Einly Lim, Jihua Chen, Pengbo Chu, Yifei Jin, Yan Wang, Xiaoliang Wang, Ying Yang, Jun Zhang, Bankole Osho, Julian F. Highmoore, Chen Zhang, Haoran Cui, S. Arthur
article en

Abstract

Fused filament fabrication has been applied to manufacture complex thermoplastic structures. However, due to the poor mechanical strength, the printed structures are typically used for prototyping purposes rather than end-use functional parts. Inspired by embedded ink writing, which produces three-dimensional architectures with enhanced mechanical properties, a molten embedded writing (MEW) method is developed in this work to print thermoplastic polymer filaments within a high-temperature support bath. The support bath is composed of organomodified montmorillonite particles and high-smoking-point sunflower oil, which offers a desired thermal environment to promote interfilament fusion, thereby enhancing the mechanical strength of as-printed structures. To demonstrate the broad and reliable application of MEW, three representative end-use parts, including orbital implants from polycaprolactone, spigots from polylactic acid for a lab-scale hydrocyclone, and sensors from thermal polyurethane, are successfully printed for repairing an orbital bone fracture, enhancing mineral particle separation, and detecting strain and force for a robotic hand, respectively.

ACS Applied Materials & InterfacesVol. 17(50)
Oak Ridge National Laboratory (US), Langley Research Center (US), University of Nevada, Reno (US), Materials Processing (United States) (US), He Eye Hospital (CN), Center for Nanophase Materials Sciences, Desert Research Institute (US), China Medical University (CN)
Openalex Percentile: Top 59%
Additive Manufacturing and 3D Printing Technologies
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