X-ray magnetic circular dichroism originating from the anisotropic magnetic dipole operator in collinear altermagnets under trigonal crystal field
We investigate the microscopic origin and spectral features of x-ray magnetic circular dichroism (XMCD) in collinear antiferromagnets with trigonal crystal fields, using $\ensuremath{\alpha}$-MnTe as a prototypical example. Although such systems exhibit zero net magnetization, we demonstrate that XMCD can emerge from the anisotropic magnetic dipole operator ${T}_{z}$, arising from quadrupolar spin distributions. By constructing a complete multipole basis and analyzing the symmetry conditions under trigonal distortion, we identify specific spin and orbital configurations that enable a finite XMCD response. Further, we employ both one-electron and multielectron models, including spin-orbit coupling and Coulomb interactions, to calculate the XMCD spectra for various ${d}^{n}$ configurations. Our findings provide theoretical benchmarks for XMCD in altermagnets and highlight the key role of orbital symmetry and magnetic anisotropy in realizing observable dichroic effects.
Authors
- Norimasa Sasabe
- Yuichi Yamasaki (ORCID: https://orcid.org/0000-0002-8560-3462)
- Yuta Ishii (ORCID: https://orcid.org/0000-0002-8957-5833)
Institutions
- Tohoku University (JP)
- National Institute for Materials Science (JP)
- RIKEN (JP)
- RIKEN Center for Emergent Matter Science (JP)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-08
- DOI
- https://doi.org/10.1103/hchg-7bq9
- Primary Topic
- Iron-based superconductors research
- Type
- article
- Field-Weighted Citation Impact
- 0.00