X-ray magnetic circular dichroism originating from the anisotropic magnetic dipole operator in collinear altermagnets under trigonal crystal field

We investigate the microscopic origin and spectral features of x-ray magnetic circular dichroism (XMCD) in collinear antiferromagnets with trigonal crystal fields, using $\ensuremath{\alpha}$-MnTe as a prototypical example. Although such systems exhibit zero net magnetization, we demonstrate that XMCD can emerge from the anisotropic magnetic dipole operator ${T}_{z}$, arising from quadrupolar spin distributions. By constructing a complete multipole basis and analyzing the symmetry conditions under trigonal distortion, we identify specific spin and orbital configurations that enable a finite XMCD response. Further, we employ both one-electron and multielectron models, including spin-orbit coupling and Coulomb interactions, to calculate the XMCD spectra for various ${d}^{n}$ configurations. Our findings provide theoretical benchmarks for XMCD in altermagnets and highlight the key role of orbital symmetry and magnetic anisotropy in realizing observable dichroic effects.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-08
DOI
https://doi.org/10.1103/hchg-7bq9
Primary Topic
Iron-based superconductors research
Type
article
Field-Weighted Citation Impact
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article

X-ray magnetic circular dichroism originating from the anisotropic magnetic dipole operator in collinear altermagnets under trigonal crystal field

Norimasa Sasabe, Yuichi Yamasaki, Yuta Ishii
Physical review. B./Physical review. B
Iron-based superconductors research
article

X-ray magnetic circular dichroism originating from the anisotropic magnetic dipole operator in collinear altermagnets under trigonal crystal field

Norimasa Sasabe, Yuichi Yamasaki, Yuta Ishii
article en

Abstract

We investigate the microscopic origin and spectral features of x-ray magnetic circular dichroism (XMCD) in collinear antiferromagnets with trigonal crystal fields, using $\ensuremath{\alpha}$-MnTe as a prototypical example. Although such systems exhibit zero net magnetization, we demonstrate that XMCD can emerge from the anisotropic magnetic dipole operator ${T}_{z}$, arising from quadrupolar spin distributions. By constructing a complete multipole basis and analyzing the symmetry conditions under trigonal distortion, we identify specific spin and orbital configurations that enable a finite XMCD response. Further, we employ both one-electron and multielectron models, including spin-orbit coupling and Coulomb interactions, to calculate the XMCD spectra for various ${d}^{n}$ configurations. Our findings provide theoretical benchmarks for XMCD in altermagnets and highlight the key role of orbital symmetry and magnetic anisotropy in realizing observable dichroic effects.

Physical review. B./Physical review. BVol. 112(22)
Tohoku University (JP), National Institute for Materials Science (JP), RIKEN (JP), RIKEN Center for Emergent Matter Science (JP)
Openalex Percentile: Top 72%
Iron-based superconductors research
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X-ray magnetic circular dichroism originating from the anisotropic magnetic dipole operator in collinear altermagnets under trigonal crystal field — Norimasa Sasabe, Yuichi Yamasaki, et al. · Physical review. B./Physical review. B (2025) | TGRS Research Map | TGRS