Magnetic and structural domain walls dynamics in a two magnetic sublattice system

The magnetic control by acoustically induced strain has driven significant research to pursue novel, ultrafast, compact, and energy-efficient electronic and spintronic devices. In this regard, magnetoelastic antiferromagnets have been highlighted as promising functional materials for this purpose. In this work, we report an experimental and phenomenological study of acoustic resonances in the two magnetic sublattices antiferromagnet ${\mathrm{NdFeO}}_{3}$, which exhibits strong interplay between magnetic and lattice degrees of freedom. The elastic properties of ${\mathrm{NdFeO}}_{3}$ are characterized through resonant ultrasound spectroscopy in the 2--300 K range. Domain-wall dynamics were studied by temperature-dependent Faraday magneto-optical imaging and AC magnetic susceptibility measurements. The results evidence the magnetoelastic coupling in ${\mathrm{NdFeO}}_{3}$, for which two different mechanisms contribute. The continuous spin reorientation transition is mirrored by the rather high acoustic losses, which correlate with the dispersion of the complex magnetic susceptibility and magnetic domain-wall dynamics. The results are compatible with the expected symmetry lowering during the spin reorientation transition and follow what is expected from a phenomenological approach. The paramagnetic ordering of the Nd sublattice under the influence of the Fe-sublattice magnetic field is found to influence the magnetoelastic properties just below the spin reorientation transition interval. This study highlights the elastic properties of ${\mathrm{NdFeO}}_{3}$, an interesting material for domain-wall motion control and local properties tailoring, which are the key for future applications in nanoscale devices.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-03
DOI
https://doi.org/10.1103/rmzj-hj3y
Primary Topic
Multiferroics and related materials
Type
article
Field-Weighted Citation Impact
0.00

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article

Magnetic and structural domain walls dynamics in a two magnetic sublattice system

M. M. Gomes, M. Mihalik, M. Mihálik, J. Agostinho Moreira et al.
Physical review. B./Physical review. B
Multiferroics and related materials
article

Magnetic and structural domain walls dynamics in a two magnetic sublattice system

M. M. Gomes, M. Mihalik, M. Mihálik, J. Agostinho Moreira, A. Kirilyuk, C. S. Davies, R. Vilarinho, Michael A. Carpenter, J.A. Paixão, Ana S. Silva
article en

Abstract

The magnetic control by acoustically induced strain has driven significant research to pursue novel, ultrafast, compact, and energy-efficient electronic and spintronic devices. In this regard, magnetoelastic antiferromagnets have been highlighted as promising functional materials for this purpose. In this work, we report an experimental and phenomenological study of acoustic resonances in the two magnetic sublattices antiferromagnet ${\mathrm{NdFeO}}_{3}$, which exhibits strong interplay between magnetic and lattice degrees of freedom. The elastic properties of ${\mathrm{NdFeO}}_{3}$ are characterized through resonant ultrasound spectroscopy in the 2--300 K range. Domain-wall dynamics were studied by temperature-dependent Faraday magneto-optical imaging and AC magnetic susceptibility measurements. The results evidence the magnetoelastic coupling in ${\mathrm{NdFeO}}_{3}$, for which two different mechanisms contribute. The continuous spin reorientation transition is mirrored by the rather high acoustic losses, which correlate with the dispersion of the complex magnetic susceptibility and magnetic domain-wall dynamics. The results are compatible with the expected symmetry lowering during the spin reorientation transition and follow what is expected from a phenomenological approach. The paramagnetic ordering of the Nd sublattice under the influence of the Fe-sublattice magnetic field is found to influence the magnetoelastic properties just below the spin reorientation transition interval. This study highlights the elastic properties of ${\mathrm{NdFeO}}_{3}$, an interesting material for domain-wall motion control and local properties tailoring, which are the key for future applications in nanoscale devices.

Physical review. B./Physical review. BVol. 112(22)
Radboud University Nijmegen (NL), Universidade do Porto (PT), Slovak Academy of Sciences (SK), University of Cambridge (GB), Institute of Experimental Physics of the Slovak Academy of Sciences (SK), Felix Scholarship (GB), Fraunhofer Institute for Manufacturing Technology and Advanced Materials (DE), HFML-FELIX (NL), University of Coimbra (PT)
Vedecká Grantová Agentúra MŠVVaŠ SR a SAV, Engineering and Physical Sciences Research Council, Natural Environment Research Council, Fundação para a Ciência e a Tecnologia
Openalex Percentile: Top 72%
Multiferroics and related materials
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