<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mi>G</mml:mi> </mml:math> -type antiferromagnetic ordering with strong anisotropic exchange interactions in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub>

Isovalent substitution of <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:msup> <a:mrow> <a:mi>Ir</a:mi> </a:mrow> <a:mrow> <a:mn>4</a:mn> <a:mo>+</a:mo> </a:mrow> </a:msup> </a:math> with <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:msup> <b:mrow> <b:mi>Sn</b:mi> </b:mrow> <b:mrow> <b:mn>4</b:mn> <b:mo>+</b:mo> </b:mrow> </b:msup> </b:math> in perovskite <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:msub> <c:mi>SrIrO</c:mi> <c:mn>3</c:mn> </c:msub> </c:math> induces a metal-insulator transition accompanied with strong antiferromagnetic ordering. We performed resonant x-ray scattering to investigate the magnetism in <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mrow> <d:msub> <d:mi>SrIr</d:mi> <d:mrow> <d:mn>0.8</d:mn> </d:mrow> </d:msub> <d:msub> <d:mi>Sn</d:mi> <d:mrow> <d:mn>0.2</d:mn> </d:mrow> </d:msub> <d:msub> <d:mi mathvariant="normal">O</d:mi> <d:mn>3</d:mn> </d:msub> </d:mrow> </d:math> . The <f:math xmlns:f="http://www.w3.org/1998/Math/MathML"> <f:mi>G</f:mi> </f:math> -type antiferromagnetic ordering with spin pointing along <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"> <g:mi>c</g:mi> </g:math> axis was fully determined by azimuth-dependent elastic scattering. Dynamical magnetic excitation spectra were measured with resonant inelastic x-ray scattering. Strong magnetic exchange interactions were observed with magnon dispersing up to <h:math xmlns:h="http://www.w3.org/1998/Math/MathML"> <h:mrow> <h:mo>∼</h:mo> <h:mn>130</h:mn> <h:mspace width="0.16em"/> <h:mi>meV</h:mi> </h:mrow> </h:math> , and the anisotropy drives a large <j:math xmlns:j="http://www.w3.org/1998/Math/MathML"> <j:mrow> <j:mo>∼</j:mo> <j:mn>50</j:mn> <j:mspace width="0.16em"/> <j:mi>meV</j:mi> </j:mrow> </j:math> gap. With these results, we discuss the paramagnetic semimetallic behavior of the undoped <l:math xmlns:l="http://www.w3.org/1998/Math/MathML"> <l:msub> <l:mi>SrIrO</l:mi> <l:mn>3</l:mn> </l:msub> </l:math> .

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Journal
Physical Review Research
Published
2025-09-30
DOI
https://doi.org/10.1103/bcp9-zg8f
Primary Topic
Magnetic and transport properties of perovskites and related materials
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article
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article

<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mi>G</mml:mi> </mml:math> -type antiferromagnetic ordering with strong anisotropic exchange interactions in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub>

Z. Islam, M. H. Upton, Haizhong Guo, Vivek Thampy et al.
Physical Review Research
Magnetic and transport properties of perovskites and related materials
article

<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mi>G</mml:mi> </mml:math> -type antiferromagnetic ordering with strong anisotropic exchange interactions in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub>

Z. Islam, M. H. Upton, Haizhong Guo, Vivek Thampy, Jiaqi Lin, Xiaoting Li, Yuan Wan, Yi‐Fan Jiang, Xiang Li, Xuerong Liu
article en

Abstract

Isovalent substitution of <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:msup> <a:mrow> <a:mi>Ir</a:mi> </a:mrow> <a:mrow> <a:mn>4</a:mn> <a:mo>+</a:mo> </a:mrow> </a:msup> </a:math> with <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:msup> <b:mrow> <b:mi>Sn</b:mi> </b:mrow> <b:mrow> <b:mn>4</b:mn> <b:mo>+</b:mo> </b:mrow> </b:msup> </b:math> in perovskite <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:msub> <c:mi>SrIrO</c:mi> <c:mn>3</c:mn> </c:msub> </c:math> induces a metal-insulator transition accompanied with strong antiferromagnetic ordering. We performed resonant x-ray scattering to investigate the magnetism in <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mrow> <d:msub> <d:mi>SrIr</d:mi> <d:mrow> <d:mn>0.8</d:mn> </d:mrow> </d:msub> <d:msub> <d:mi>Sn</d:mi> <d:mrow> <d:mn>0.2</d:mn> </d:mrow> </d:msub> <d:msub> <d:mi mathvariant="normal">O</d:mi> <d:mn>3</d:mn> </d:msub> </d:mrow> </d:math> . The <f:math xmlns:f="http://www.w3.org/1998/Math/MathML"> <f:mi>G</f:mi> </f:math> -type antiferromagnetic ordering with spin pointing along <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"> <g:mi>c</g:mi> </g:math> axis was fully determined by azimuth-dependent elastic scattering. Dynamical magnetic excitation spectra were measured with resonant inelastic x-ray scattering. Strong magnetic exchange interactions were observed with magnon dispersing up to <h:math xmlns:h="http://www.w3.org/1998/Math/MathML"> <h:mrow> <h:mo>∼</h:mo> <h:mn>130</h:mn> <h:mspace width="0.16em"/> <h:mi>meV</h:mi> </h:mrow> </h:math> , and the anisotropy drives a large <j:math xmlns:j="http://www.w3.org/1998/Math/MathML"> <j:mrow> <j:mo>∼</j:mo> <j:mn>50</j:mn> <j:mspace width="0.16em"/> <j:mi>meV</j:mi> </j:mrow> </j:math> gap. With these results, we discuss the paramagnetic semimetallic behavior of the undoped <l:math xmlns:l="http://www.w3.org/1998/Math/MathML"> <l:msub> <l:mi>SrIrO</l:mi> <l:mn>3</l:mn> </l:msub> </l:math> .

Physical Review ResearchVol. 7(4)
Argonne National Laboratory (US), Chinese Academy of Sciences (CN), SLAC National Accelerator Laboratory (US), ShanghaiTech University (CN), Westlake University (CN), Zhengzhou University (CN), Henan Academy of Sciences (CN), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ)
Openalex Percentile: Top 73%
Magnetic and transport properties of perovskites and related materials
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