Nature of quantum criticality in the Ising ferromagnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>TbV</mml:mi> <mml:mn>6</mml:mn> </mml:msub> <mml:msub> <mml:mi>Sn</mml:mi> <mml:mn>6</mml:mn> </mml:msub> <

<a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi>TbV</a:mi> <a:mn>6</a:mn> </a:msub> <a:msub> <a:mi>Sn</a:mi> <a:mn>6</a:mn> </a:msub> </a:mrow> </a:math> is a topological metal where ferromagnetic Tb ions with strong uniaxial magnetic anisotropy interact with V kagome layers. Inelastic neutron scattering (INS) measurements show that the Tb ions adopt an Ising doublet ground state. Here, we consider whether a transverse magnetic field can drive <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:mrow> <b:msub> <b:mi>TbV</b:mi> <b:mn>6</b:mn> </b:msub> <b:msub> <b:mi>Sn</b:mi> <b:mn>6</b:mn> </b:msub> </b:mrow> </b:math> toward a quantum critical point, providing a rare example of transverse-field Ising criticality in a metallic compound. High-field magnetization measurements reveal a first-order-like spin-reorientation transition at 25.6 T. Our INS-based magnetic model finds that this is caused by an avoided crossing of an excited-state singlet with the ground-state doublet. Surprisingly, our model predicts that quantum critical and tricritical points are accessible within the range of experimentally determined model parameters and may be reached by varying the direction of an applied magnetic field.

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Publication Details

Journal
Physical Review Research
Published
2025-10-17
DOI
https://doi.org/10.1103/jlnl-y35t
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
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Nature of quantum criticality in the Ising ferromagnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>TbV</mml:mi> <mml:mn>6</mml:mn> </mml:msub> <mml:msub> <mml:mi>Sn</mml:mi> <mml:mn>6</mml:mn> </mml:msub> <

John Singleton, Daniel M. Pajerowski, Joanna Bławat, R. McDonald et al.
Physical Review Research
Topological Materials and Phenomena
article

Nature of quantum criticality in the Ising ferromagnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>TbV</mml:mi> <mml:mn>6</mml:mn> </mml:msub> <mml:msub> <mml:mi>Sn</mml:mi> <mml:mn>6</mml:mn> </mml:msub> <

John Singleton, Daniel M. Pajerowski, Joanna Bławat, R. McDonald, P. C. Canfield, Y. Lee, Liqin Ke, Rebecca Flint, Tianxiong Han, R. J. McQueeney, R. D. McKenzie, Tyler J. Slade, Bing Li
article en

Abstract

<a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi>TbV</a:mi> <a:mn>6</a:mn> </a:msub> <a:msub> <a:mi>Sn</a:mi> <a:mn>6</a:mn> </a:msub> </a:mrow> </a:math> is a topological metal where ferromagnetic Tb ions with strong uniaxial magnetic anisotropy interact with V kagome layers. Inelastic neutron scattering (INS) measurements show that the Tb ions adopt an Ising doublet ground state. Here, we consider whether a transverse magnetic field can drive <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:mrow> <b:msub> <b:mi>TbV</b:mi> <b:mn>6</b:mn> </b:msub> <b:msub> <b:mi>Sn</b:mi> <b:mn>6</b:mn> </b:msub> </b:mrow> </b:math> toward a quantum critical point, providing a rare example of transverse-field Ising criticality in a metallic compound. High-field magnetization measurements reveal a first-order-like spin-reorientation transition at 25.6 T. Our INS-based magnetic model finds that this is caused by an avoided crossing of an excited-state singlet with the ground-state doublet. Surprisingly, our model predicts that quantum critical and tricritical points are accessible within the range of experimentally determined model parameters and may be reached by varying the direction of an applied magnetic field.

Physical Review ResearchVol. 7(4)
Oak Ridge National Laboratory (US), Los Alamos National Laboratory (US), Iowa State University (US), Ames National Laboratory (US), National High Magnetic Field Laboratory (US), University of Virginia (US)
Openalex Percentile: Top 70%
Topological Materials and Phenomena
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