Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal

We report coherent X-ray imaging of antiferromagnetic (AFM) domains and domain walls in MnBi<sub>2</sub>Te4, an intrinsic AFM topological insulator. This technique enables direct visualization of domain morphology without reconstruction algorithms, allowing us to resolve antiphase domain walls as distinct dark lines arising from the A-type AFM structure. The wall width is determined to be 550(30) nm, in good agreement with earlier magnetic force microscopy results. The temperature dependence of the AFM order parameter extracted from our images closely follows previous neutron scattering data. Remarkably, however, we find a pronounced hysteresis in the evolution of domains and domain walls: upon cooling, dynamic reorganizations occur within a narrow ∼1 K interval below TN, whereas upon warming, the domain configuration remains largely unchanged until AFM order disappears. These findings reveal a complex energy landscape in MnBi2Te4, governed by the interplay of exchange, anisotropy, and domain-wall energies, and underscore the critical role of AFM domain-wall dynamics in shaping its physical properties. These sharply defined and hysteretically evolving walls may provide a controllable AFM texture in MnBi2Te4, hinting at potential use in low-power spintronic devices based on domain-wall dynamics.

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Publication Details

Journal
Materials
Published
2025-11-26
DOI
https://doi.org/10.3390/ma18235337
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
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article

Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal

M. G. Kim, C. Mazzoli, Luke Burgard, Lillian Rutowski et al.
Materials
Topological Materials and Phenomena
article

Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal

M. G. Kim, C. Mazzoli, Luke Burgard, Lillian Rutowski, Starr Boney
article en

Abstract

We report coherent X-ray imaging of antiferromagnetic (AFM) domains and domain walls in MnBi<sub>2</sub>Te4, an intrinsic AFM topological insulator. This technique enables direct visualization of domain morphology without reconstruction algorithms, allowing us to resolve antiphase domain walls as distinct dark lines arising from the A-type AFM structure. The wall width is determined to be 550(30) nm, in good agreement with earlier magnetic force microscopy results. The temperature dependence of the AFM order parameter extracted from our images closely follows previous neutron scattering data. Remarkably, however, we find a pronounced hysteresis in the evolution of domains and domain walls: upon cooling, dynamic reorganizations occur within a narrow ∼1 K interval below TN, whereas upon warming, the domain configuration remains largely unchanged until AFM order disappears. These findings reveal a complex energy landscape in MnBi2Te4, governed by the interplay of exchange, anisotropy, and domain-wall energies, and underscore the critical role of AFM domain-wall dynamics in shaping its physical properties. These sharply defined and hysteretically evolving walls may provide a controllable AFM texture in MnBi2Te4, hinting at potential use in low-power spintronic devices based on domain-wall dynamics.

MaterialsVol. 18(23)
Brookhaven National Laboratory (US), University of Wisconsin–Milwaukee (US)
U.S. Department of Energy, University of Wisconsin-Milwaukee, Office of Science, Laboratory Directed Research and Development, Brookhaven National Laboratory
Openalex Percentile: Top 71%
Topological Materials and Phenomena
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Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal — M. G. Kim, C. Mazzoli, et al. · Materials (2025) | TGRS Research Map | TGRS