Catalytic activity of supported Cu-Mn/fly ash geopolymer for the oxidative removal of toluene

This study successfully developed Cu-Mn supported catalysts on fly ash geopolymer for the oxidative removal of toluene. The surface characteristics and catalytic performance of catalysts were systematically investigated in this paper. It was found that the Cu/Mn ratio plays a crucial role in determining the catalysts' performance, with the Geo-3 catalyst showing the highest toluene conversion rate of 90% at 296 ℃. The catalyst also exhibited the lowest activation energy of 123.0 kJ/mol, indicating its superior catalytic efficiency. The findings not only contribute to the development of cost-effective and efficient catalysts for VOCs degradation but also provide valuable insights into the influence of the Cu/Mn ratio on the catalytic properties of geopolymer-supported Cu-Mn catalysts. This research offers a promising approach for the abatement of VOCs in industrial emissions.

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Publication Details

Journal
Scientific Reports
Published
2025-11-27
DOI
https://doi.org/10.1038/s41598-025-07359-x
Primary Topic
Catalytic Processes in Materials Science
Type
article
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article

Catalytic activity of supported Cu-Mn/fly ash geopolymer for the oxidative removal of toluene

Qingqing Guan, Mengqi Zhao, Xiaoyang Liang, Jiawei Feng et al.
Scientific Reports
Catalytic Processes in Materials Science
article

Catalytic activity of supported Cu-Mn/fly ash geopolymer for the oxidative removal of toluene

Qingqing Guan, Mengqi Zhao, Xiaoyang Liang, Jiawei Feng, Dejun Chen, Hao Yuan
article en

Abstract

This study successfully developed Cu-Mn supported catalysts on fly ash geopolymer for the oxidative removal of toluene. The surface characteristics and catalytic performance of catalysts were systematically investigated in this paper. It was found that the Cu/Mn ratio plays a crucial role in determining the catalysts' performance, with the Geo-3 catalyst showing the highest toluene conversion rate of 90% at 296 ℃. The catalyst also exhibited the lowest activation energy of 123.0 kJ/mol, indicating its superior catalytic efficiency. The findings not only contribute to the development of cost-effective and efficient catalysts for VOCs degradation but also provide valuable insights into the influence of the Cu/Mn ratio on the catalytic properties of geopolymer-supported Cu-Mn catalysts. This research offers a promising approach for the abatement of VOCs in industrial emissions.

Scientific ReportsVol. 15(1)
Xinjiang Uygur Autonomous Region Product Quality Supervision and Inspection Institute (CN), National Institute of Clean and Low-Carbon Energy (CN), Xinjiang New Energy Research Institute (China) (CN), Xinjiang University (CN)
Openalex Percentile: Top 70%
Catalytic Processes in Materials Science
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Catalytic activity of supported Cu-Mn/fly ash geopolymer for the oxidative removal of toluene — Qingqing Guan, Mengqi Zhao, et al. · Scientific Reports (2025) | TGRS Research Map | TGRS