Aerogel-inspired interfacial engineering of metal–organic framework and black phosphorus heterojunction for enhanced CO <sub>2</sub> photocatalytic reduction
Photocatalytic reduction of CO<sub>2</sub> to value-added products shows promise for addressing energy and environmental challenges, but is constrained by inefficient charge separation and light utilization. We develop an aerogel-inspired mechanochemical strategy to fabricate NH<sub>2</sub>-UiO-66 and black phosphorus heterojunctions that feature robust interfacial coupling and stabilization of key intermediates to promote CO<sub>2</sub>-to-CO conversion.
Authors
- Zunbin Duan (ORCID: https://orcid.org/0000-0002-7190-650X)
- Jenaidullah Batur (ORCID: https://orcid.org/0000-0002-0460-9548)
- Guanglei Zhang (ORCID: https://orcid.org/0000-0002-2617-9673)
- Yanfang Li (ORCID: https://orcid.org/0000-0003-2761-0282)
- Rui Li (ORCID: https://orcid.org/0000-0003-4379-8801)
- Huiming Zhang (ORCID: https://orcid.org/0009-0007-1695-8511)
Institutions
- Vaughn College of Aeronautics and Technology (US)
- Shandong University (CN)
- University of Jinan (CN)
- Beijing University of Technology (CN)
Publication Details
- Journal
- Chemical Communications
- Published
- 2025-11-27
- DOI
- https://doi.org/10.1039/d5cc06050h
- Primary Topic
- Metal-Organic Frameworks: Synthesis and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00