High- <i>Q</i> Resonances in Hybrid Plasmonic–Photonic Metasurfaces

Plasmonic systems supporting resonances with a high quality (<i>Q</i>) factor are highly desirable for applications such as optical sensing and nanolasing. However, this goal is hindered by radiative loss and Ohmic loss. This paper reports a hybrid plasmonic-photonic system that supports multiple high-<i>Q</i> resonances in the short-wave near-infrared regime, which are associated with either at-Γ or off-Γ bound states in the continuum (BICs). By engineering the hybridization between a dielectric slab waveguide and a plasmonic nanoparticle lattice, BICs can form via symmetry incompatibility or destructive interference. Concurrently, the enhanced electric fields are distributed away from the lossy metal, thus enabling high-<i>Q</i> optical resonances in plasmonic systems. Experimentally, we fabricate two-dimensional silver nanoparticle arrays embedded within a dielectric slab waveguide. The highest <i>Q</i> factor observed is ∼2140 at λ = 985 nm. In addition, by utilizing such nonlocal resonant modes near the BIC condition at the excitation wavelength, we demonstrate significantly enhanced upconversion luminescence from doped erbium ions. This type of metasurface thus offers prospects for future studies where a high <i>Q</i> factor and enhanced light-matter interactions are required.

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Publication Details

Journal
The Journal of Physical Chemistry Letters
Published
2025-11-26
DOI
https://doi.org/10.1021/acs.jpclett.5c02920
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
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article

High- Q Resonances in Hybrid Plasmonic–Photonic Metasurfaces

Xianyu Ao, C. L. Bai, Xiao-Jun Bi
The Journal of Physical Chemistry Letters
Plasmonic and Surface Plasmon Research
article

High- Q Resonances in Hybrid Plasmonic–Photonic Metasurfaces

Xianyu Ao, C. L. Bai, Xiao-Jun Bi
article en

Abstract

Plasmonic systems supporting resonances with a high quality (<i>Q</i>) factor are highly desirable for applications such as optical sensing and nanolasing. However, this goal is hindered by radiative loss and Ohmic loss. This paper reports a hybrid plasmonic-photonic system that supports multiple high-<i>Q</i> resonances in the short-wave near-infrared regime, which are associated with either at-Γ or off-Γ bound states in the continuum (BICs). By engineering the hybridization between a dielectric slab waveguide and a plasmonic nanoparticle lattice, BICs can form via symmetry incompatibility or destructive interference. Concurrently, the enhanced electric fields are distributed away from the lossy metal, thus enabling high-<i>Q</i> optical resonances in plasmonic systems. Experimentally, we fabricate two-dimensional silver nanoparticle arrays embedded within a dielectric slab waveguide. The highest <i>Q</i> factor observed is ∼2140 at λ = 985 nm. In addition, by utilizing such nonlocal resonant modes near the BIC condition at the excitation wavelength, we demonstrate significantly enhanced upconversion luminescence from doped erbium ions. This type of metasurface thus offers prospects for future studies where a high <i>Q</i> factor and enhanced light-matter interactions are required.

The Journal of Physical Chemistry LettersVol. 16(49)
Shandong Normal University (CN), Applications Research (United States) (US)
Openalex Percentile: Top 64%
Plasmonic and Surface Plasmon Research
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