Tuning the Decay Length of Long-Range Photocurrent in Weyl Semimetals by Engineering the Weighting Field
In conventional materials, symmetry breaking induced by spatial inhomogeneities typically confines self-powered photocurrents to edges, corners, or interfaces. In this work, we observe long-range photocurrents with multidomain patterns extending from the contacts into the interior of homogeneous Weyl semimetals (WTe<sub>2</sub> and TaIrTe<sub>4</sub>) at room temperature. It is revealed that the long-range photocurrent is approximately proportional to the anisotropic divergence of the weighting field ((<b>σS</b>∇)·<b>E</b>). By increasing the conductivity anisotropy or enlarging the angle between the material's <i>a-</i>axis and the channel direction, the gradient of (<b>σS</b>∇)·<b>E</b> along the <i>a</i>-axis is reduced, and the decay length of the long-range photocurrent (<i>L</i><sub>d</sub>) is substantially increased. As a result, a large <i>L</i><sub>d</sub> of up to 20.5 μm is achieved in a TaIrTe<sub>4</sub> device with the <i>a</i>-axis oriented perpendicular to the channel direction, far exceeding typical photocurrent decay lengths observed in conventional low-dimensional materials.
Authors
- Tianyuan Cui
- Xu Dai (ORCID: https://orcid.org/0009-0006-5257-5406)
- Yujie Zhang (ORCID: https://orcid.org/0000-0002-5989-4892)
- Ye Tao (ORCID: https://orcid.org/0000-0003-4814-767X)
- Jiajun Ma (ORCID: https://orcid.org/0000-0002-1384-1445)
- Huiming Luo (ORCID: https://orcid.org/0000-0002-4431-8454)
- Yonghao Bu
- Mengdie Shi (ORCID: https://orcid.org/0000-0001-7149-8094)
- Jing Zhou (ORCID: https://orcid.org/0000-0003-0190-7715)
- Jie Deng (ORCID: https://orcid.org/0000-0003-1081-7869)
- Wei Zhang (ORCID: https://orcid.org/0000-0003-2577-9551)
- Xiaoshuang Chen (ORCID: https://orcid.org/0000-0003-0131-9454)
- Junwei Huang
- Jie Pan (ORCID: https://orcid.org/0009-0000-0145-6104)
- Lin Wang (ORCID: https://orcid.org/0000-0003-3033-4792)
- Ruowen Wang
Institutions
- Nanjing Tech University (CN)
- Shanghai Institute of Technical Physics (CN)
- Infrared Laboratories (United States) (US)
- The Synergetic Innovation Center for Advanced Materials (CN)
- University of Chinese Academy of Sciences (CN)
- State Key Laboratory of Infrared Physics
Publication Details
- Journal
- Nano Letters
- Published
- 2025-11-26
- DOI
- https://doi.org/10.1021/acs.nanolett.5c05323
- Primary Topic
- Topological Materials and Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 0.00