Tuning the Decay Length of Long-Range Photocurrent in Weyl Semimetals by Engineering the Weighting Field

In conventional materials, symmetry breaking induced by spatial inhomogeneities typically confines self-powered photocurrents to edges, corners, or interfaces. In this work, we observe long-range photocurrents with multidomain patterns extending from the contacts into the interior of homogeneous Weyl semimetals (WTe<sub>2</sub> and TaIrTe<sub>4</sub>) at room temperature. It is revealed that the long-range photocurrent is approximately proportional to the anisotropic divergence of the weighting field ((<b>σS</b>∇)·<b>E</b>). By increasing the conductivity anisotropy or enlarging the angle between the material's <i>a-</i>axis and the channel direction, the gradient of (<b>σS</b>∇)·<b>E</b> along the <i>a</i>-axis is reduced, and the decay length of the long-range photocurrent (<i>L</i><sub>d</sub>) is substantially increased. As a result, a large <i>L</i><sub>d</sub> of up to 20.5 μm is achieved in a TaIrTe<sub>4</sub> device with the <i>a</i>-axis oriented perpendicular to the channel direction, far exceeding typical photocurrent decay lengths observed in conventional low-dimensional materials.

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Publication Details

Journal
Nano Letters
Published
2025-11-26
DOI
https://doi.org/10.1021/acs.nanolett.5c05323
Primary Topic
Topological Materials and Phenomena
Type
article
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article

Tuning the Decay Length of Long-Range Photocurrent in Weyl Semimetals by Engineering the Weighting Field

Tianyuan Cui, Xu Dai, Yujie Zhang, Ye Tao et al.
Nano Letters
Topological Materials and Phenomena
article

Tuning the Decay Length of Long-Range Photocurrent in Weyl Semimetals by Engineering the Weighting Field

Tianyuan Cui, Xu Dai, Yujie Zhang, Ye Tao, Jiajun Ma, Huiming Luo, Yonghao Bu, Mengdie Shi, Jing Zhou, Jie Deng, Wei Zhang, Xiaoshuang Chen, Junwei Huang, Jie Pan, Lin Wang, Ruowen Wang
article en

Abstract

In conventional materials, symmetry breaking induced by spatial inhomogeneities typically confines self-powered photocurrents to edges, corners, or interfaces. In this work, we observe long-range photocurrents with multidomain patterns extending from the contacts into the interior of homogeneous Weyl semimetals (WTe<sub>2</sub> and TaIrTe<sub>4</sub>) at room temperature. It is revealed that the long-range photocurrent is approximately proportional to the anisotropic divergence of the weighting field ((<b>σS</b>∇)·<b>E</b>). By increasing the conductivity anisotropy or enlarging the angle between the material's <i>a-</i>axis and the channel direction, the gradient of (<b>σS</b>∇)·<b>E</b> along the <i>a</i>-axis is reduced, and the decay length of the long-range photocurrent (<i>L</i><sub>d</sub>) is substantially increased. As a result, a large <i>L</i><sub>d</sub> of up to 20.5 μm is achieved in a TaIrTe<sub>4</sub> device with the <i>a</i>-axis oriented perpendicular to the channel direction, far exceeding typical photocurrent decay lengths observed in conventional low-dimensional materials.

Nano LettersVol. 25(50)
Nanjing Tech University (CN), Shanghai Institute of Technical Physics (CN), Infrared Laboratories (United States) (US), The Synergetic Innovation Center for Advanced Materials (CN), University of Chinese Academy of Sciences (CN), State Key Laboratory of Infrared Physics
Openalex Percentile: Top 71%
Topological Materials and Phenomena
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