Battery SOH estimation based on thermodynamic parameters from an electrochemical fractional-order model and LSTM

Accurate state of health (SOH) estimation is vital for lithium-ion battery safety and performance. Since SOH cannot be directly measured, traditional methods rely on external features or models but often suffer from low interpretability and complex modeling. This study proposes a physics-inspired deep learning method for SOH estimation, which combines battery mechanism models with deep learning to effectively incorporate physical insights and improve predictive performance. Thermodynamic parameters from an electrochemical fractional-order model are fed into a long short-term memory (LSTM) network to map features to SOH, enabling high-precision estimation. Compared with four other machine learning methods, LSTM achieved the best performance, with an average root-mean-square error of 0.70% and a minimum error of 0.21% across eight validation batteries. The use of thermodynamic parameters improved estimation accuracy by 3.36 times compared to traditional features like incremental capacity curves and ohmic resistance. This approach integrates physical modeling with data-driven methods, enabling high-precision battery management.

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Publication Details

Journal
iScience
Published
2025-11-26
DOI
https://doi.org/10.1016/j.isci.2025.114234
Primary Topic
Advanced Battery Technologies Research
Type
article
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article

Battery SOH estimation based on thermodynamic parameters from an electrochemical fractional-order model and LSTM

Peipei Meng, Guorong Zhu, Jing V. Wang, Jianqiang Kang et al.
iScience
Advanced Battery Technologies Research
article

Battery SOH estimation based on thermodynamic parameters from an electrochemical fractional-order model and LSTM

Peipei Meng, Guorong Zhu, Jing V. Wang, Jianqiang Kang, Qian Wang, Yi Liu
article en

Abstract

Accurate state of health (SOH) estimation is vital for lithium-ion battery safety and performance. Since SOH cannot be directly measured, traditional methods rely on external features or models but often suffer from low interpretability and complex modeling. This study proposes a physics-inspired deep learning method for SOH estimation, which combines battery mechanism models with deep learning to effectively incorporate physical insights and improve predictive performance. Thermodynamic parameters from an electrochemical fractional-order model are fed into a long short-term memory (LSTM) network to map features to SOH, enabling high-precision estimation. Compared with four other machine learning methods, LSTM achieved the best performance, with an average root-mean-square error of 0.70% and a minimum error of 0.21% across eight validation batteries. The use of thermodynamic parameters improved estimation accuracy by 3.36 times compared to traditional features like incremental capacity curves and ohmic resistance. This approach integrates physical modeling with data-driven methods, enabling high-precision battery management.

iScienceVol. 29(1)
Wuhan University of Technology (CN), Hubei University of Automotive Technology (CN)
Openalex Percentile: Top 60%
Advanced Battery Technologies Research
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