Correlation-promoted electron-phonon coupling and superconductivity in bulk FeSe

Electron-phonon coupling (EPC) plays an important role in FeSe, yet theoretical predictions have struggled to reconcile with experiments on doping- and pressure-dependent superconductivity. Here, we employ dynamical mean-field theory to investigate correlation-corrected EPC in FeSe under carrier doping and pressure. By incorporating correlation-corrected EPC strength and applying the Migdal-Eliashberg formalism for phonon-mediated superconductivity, we predict superconducting transition temperatures ${T}_{c}$ that closely match experiments and reproduce the observed doping- and pressure-dependent trends. We further find that the electronic correlation strength, characterized by the bandwidth near the Fermi level, shows an opposite trend to ${T}_{c}$, in contrast to EPC. Our work demonstrates the consistency of the correlation-promoted EPC and ${T}_{c}$ over a range of experimental conditions, which suggests that superconductivity in FeSe may originate primarily from correlation-promoted electron-phonon coupling.

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Publication Details

Journal
Physical Review Materials
Published
2025-11-21
DOI
https://doi.org/10.1103/9qx8-7q4x
Primary Topic
Iron-based superconductors research
Type
article
Field-Weighted Citation Impact
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article

Correlation-promoted electron-phonon coupling and superconductivity in bulk FeSe

Sheng Meng, Shiqi Hu, Yang Yang, Lan-Lin Du et al.
Physical Review Materials
Iron-based superconductors research
article

Correlation-promoted electron-phonon coupling and superconductivity in bulk FeSe

Sheng Meng, Shiqi Hu, Yang Yang, Lan-Lin Du, XIANGLONG BU
article en

Abstract

Electron-phonon coupling (EPC) plays an important role in FeSe, yet theoretical predictions have struggled to reconcile with experiments on doping- and pressure-dependent superconductivity. Here, we employ dynamical mean-field theory to investigate correlation-corrected EPC in FeSe under carrier doping and pressure. By incorporating correlation-corrected EPC strength and applying the Migdal-Eliashberg formalism for phonon-mediated superconductivity, we predict superconducting transition temperatures ${T}_{c}$ that closely match experiments and reproduce the observed doping- and pressure-dependent trends. We further find that the electronic correlation strength, characterized by the bandwidth near the Fermi level, shows an opposite trend to ${T}_{c}$, in contrast to EPC. Our work demonstrates the consistency of the correlation-promoted EPC and ${T}_{c}$ over a range of experimental conditions, which suggests that superconductivity in FeSe may originate primarily from correlation-promoted electron-phonon coupling.

Physical Review MaterialsVol. 9(11)
Chinese Academy of Sciences (CN), Songshan Lake Materials Laboratory (CN), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), Institute of Physics (CN), University of Chinese Academy of Sciences (CN)
Openalex Percentile: Top 74%
Iron-based superconductors research
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Correlation-promoted electron-phonon coupling and superconductivity in bulk FeSe — Sheng Meng, Shiqi Hu, et al. · Physical Review Materials (2025) | TGRS Research Map | TGRS