High-order strong-coupling expansion for x-ray absorption on a dynamically screened impurity
Time-resolved x-ray absorption can reveal the dynamical screening of the local Coulomb interaction in strongly correlated photodoped materials. Here, we focus on the theoretical prediction of x-ray absorption in the presence of dynamical screening using the strong-coupling expansion, i.e., an expansion around the isolated absorption site in terms of the retarded interaction. The evaluation of higher-order diagrams is made numerically feasible by an approach based on the decomposition of the retarded interaction into complex exponentials. With this, we evaluate the strong-coupling series to third order on an electron-boson model of Holstein type. We demonstrate that in relevant coupling regimes, even low orders of the strong-coupling expansion can give a significant correction over the previously used lowest-order approximation.
Authors
- Eva Paprotzki (ORCID: https://orcid.org/0009-0008-2368-2573)
- MARTIN C. ECKSTEIN (ORCID: https://orcid.org/0000-0003-0124-5408)
Institutions
- Universität Hamburg (DE)
- Hamburg Centre for Ultrafast Imaging
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-21
- DOI
- https://doi.org/10.1103/bl6z-14m9
- Citations
- 1
- Primary Topic
- Advanced X-ray Imaging Techniques
- Type
- article
- Field-Weighted Citation Impact
- 1.88