Cyclotron resonance in a kagome spin liquid candidate material

We propose cyclotron resonance as an optical probe for emergent fractionalized excitations in $\mathrm{U}(1)$ quantum spin liquids, focusing on kagome antiferromagnets. In contrast to conventional systems, where cyclotron resonance directly couples to charged carriers, spinons in spin liquids are charge-neutral and interact only through an emergent gauge field, making direct probing challenging. We identify two key mechanisms by which an external physical electromagnetic field induces emergent electric and magnetic fields, enabling indirect coupling to spinons. Using these mechanisms, we compute the absorption rate of the cyclotron resonance response for Dirac spinons forming Landau levels. Our analysis shows that, although the absorption per layer is small, the absence of a skin-depth limitation in insulating spin liquids allows for cumulative absorption comparable to graphene in realistic sample sizes for the recently discovered spin-liquid candidate material ${\mathrm{YCu}}_{3}{(\mathrm{OH})}_{6}{\mathrm{Br}}_{2}[\mathrm{Br}{}_{1\ensuremath{-}y}{(\mathrm{OH})}_{y}]$. Our proposed cyclotron-resonance measurement is a decisive, practical test for spinon Landau levels, providing quantitative expectations where clear experimental evidence has so far been lacking.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-11-20
DOI
https://doi.org/10.1103/qgr3-5m54
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
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article

Cyclotron resonance in a kagome spin liquid candidate material

Patrick A. Lee, Byungmin Kang
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
article

Cyclotron resonance in a kagome spin liquid candidate material

Patrick A. Lee, Byungmin Kang
article en

Abstract

We propose cyclotron resonance as an optical probe for emergent fractionalized excitations in $\mathrm{U}(1)$ quantum spin liquids, focusing on kagome antiferromagnets. In contrast to conventional systems, where cyclotron resonance directly couples to charged carriers, spinons in spin liquids are charge-neutral and interact only through an emergent gauge field, making direct probing challenging. We identify two key mechanisms by which an external physical electromagnetic field induces emergent electric and magnetic fields, enabling indirect coupling to spinons. Using these mechanisms, we compute the absorption rate of the cyclotron resonance response for Dirac spinons forming Landau levels. Our analysis shows that, although the absorption per layer is small, the absence of a skin-depth limitation in insulating spin liquids allows for cumulative absorption comparable to graphene in realistic sample sizes for the recently discovered spin-liquid candidate material ${\mathrm{YCu}}_{3}{(\mathrm{OH})}_{6}{\mathrm{Br}}_{2}[\mathrm{Br}{}_{1\ensuremath{-}y}{(\mathrm{OH})}_{y}]$. Our proposed cyclotron-resonance measurement is a decisive, practical test for spinon Landau levels, providing quantitative expectations where clear experimental evidence has so far been lacking.

Physical review. B./Physical review. BVol. 112(20)
Massachusetts Institute of Technology (US)
Openalex Percentile: Top 77%
Advanced Condensed Matter Physics
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