Magneto-optical spectroscopy based on pump-probe strobe light
We demonstrate a pump-probe strobe light spectroscopy for sensitive detection of magneto-optical dynamics in the context of hybrid magnonics. The technique uses a combinatorial microwave-optical pump-probe scheme, leveraging both the high-energy resolution of microwaves and high-efficiency detection using optical photons. In contrast with conventional stroboscopy using continuous-wave light, we apply microwave and optical pulses with varying pulse widths, and demonstrate magneto-optical detection of magnetization dynamics in ${\mathrm{Y}}_{3}{\mathrm{Fe}}_{5}{\mathrm{O}}_{12}$ films. The detected magneto-optical signals depend strongly on the characteristics of both the microwave and the optical pulses, as well as their relative time delays. We show that good magneto-optical sensitivity and coherent stroboscopic character are maintained, even at a microwave pump pulse of 1.5 ns and an optical probe pulse of 80 ps, under a 7 MHz clock rate, corresponding to a pump-probe footprint of approximately $1\mathrm{%}$ in one detection cycle. Our results show that time-dependent strobe light measurement of magnetization dynamics can be achieved in the gigahertz frequency range under a pump-probe detection scheme.
Authors
- V. Novosad (ORCID: https://orcid.org/0000-0003-2127-2374)
- Yujie Zhu (ORCID: https://orcid.org/0000-0002-1414-2590)
- Wencan Jin (ORCID: https://orcid.org/0000-0002-5087-8562)
- Jia‐Mian Hu (ORCID: https://orcid.org/0000-0002-7579-6440)
- Shihao Zhou
- F. Tsui (ORCID: https://orcid.org/0000-0002-8769-5540)
- Yuzan Xiong (ORCID: https://orcid.org/0009-0005-6151-1300)
- Chunli Tang (ORCID: https://orcid.org/0000-0001-8252-3195)
- Wei Zhang (ORCID: https://orcid.org/0000-0002-5878-3090)
- Dali Sun (ORCID: https://orcid.org/0000-0003-4662-3265)
- Yi Li (ORCID: https://orcid.org/0000-0002-3207-7147)
- Junming Wu
- Binbin Yang (ORCID: https://orcid.org/0000-0001-7755-6072)
- Rui Sun (ORCID: https://orcid.org/0000-0003-1972-6541)
- Ingrid E. Russell (ORCID: https://orcid.org/0009-0003-0576-7497)
Institutions
- University of North Carolina at Chapel Hill (US)
- Argonne National Laboratory (US)
- University of Wisconsin–Madison (US)
- North Carolina State University (US)
- North Carolina Agricultural and Technical State University (US)
- Auburn University (US)
Publication Details
- Journal
- Physical Review Applied
- Published
- 2025-11-20
- DOI
- https://doi.org/10.1103/dj9z-347y
- Citations
- 1
- Primary Topic
- Magneto-Optical Properties and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.73