Investigation of kinetic inductance and microwave loss in thin-film TaCxN1−x superconducting resonators
The promise of tantalum for realizing superconducting quantum devices has generated interest in its compound films, particularly nitrides. Among these, cubic-phase tantalum carbonitride (TaCxN1−x) offers reduced susceptibility to oxidation and a high critical temperature, yet its microwave properties remain largely unexplored. Here, we investigate plasma-enhanced atomic layer deposition of cubic-phase TaCxN1−x thin films for superconducting microwave circuits. Structural and transport measurements reveal nanocrystalline morphology with sub-10 nm grains and superconductivity in the dirty limit. Coplanar waveguide resonators exhibit moderately high kinetic inductance (16.8 pH/sq for 30 nm films) with potential for enhancement through dimensional scaling. The films also support high internal quality factors exceeding 105 at 50 mK in the single-photon regime, comparable to granular aluminum. Loss analysis identifies the two-level systems as the dominant limiting mechanism, with potential for further reduction through interface engineering. These results establish atomic layer deposited TaCxN1−x as a promising material for scalable, low-loss, high-inductance superconducting circuits.
Authors
- Dmytro Nykypanchuk (ORCID: https://orcid.org/0000-0002-0461-3467)
- Xiao Tong (ORCID: https://orcid.org/0000-0002-5567-9677)
- Sooyeon Hwang (ORCID: https://orcid.org/0000-0001-5606-6728)
- Matthew LaHaye (ORCID: https://orcid.org/0000-0003-1911-0704)
- M. D. Nguyen (ORCID: https://orcid.org/0000-0001-9414-6083)
- Davood Shahrjerdi (ORCID: https://orcid.org/0000-0002-5955-1830)
- Moeid Jamalzadeh (ORCID: https://orcid.org/0009-0003-4550-1108)
- M. R. Perez (ORCID: https://orcid.org/0009-0006-0041-6788)
- Christopher Nadeau (ORCID: https://orcid.org/0000-0002-1944-9735)
- Iliya Shiravand (ORCID: https://orcid.org/0009-0006-4133-9723)
Institutions
- United States Air Force Research Laboratory (US)
- Booz Allen Hamilton (United States) (US)
- State University of New York (US)
- Brookhaven National Laboratory (US)
- New York University (US)
Publication Details
- Journal
- Applied Physics Letters
- Published
- 2025-11-10
- DOI
- https://doi.org/10.1063/5.0300902
- Primary Topic
- Diamond and Carbon-based Materials Research
- Type
- article
- Field-Weighted Citation Impact
- 0.00