Investigation of kinetic inductance and microwave loss in thin-film TaCxN1−x superconducting resonators

The promise of tantalum for realizing superconducting quantum devices has generated interest in its compound films, particularly nitrides. Among these, cubic-phase tantalum carbonitride (TaCxN1−x) offers reduced susceptibility to oxidation and a high critical temperature, yet its microwave properties remain largely unexplored. Here, we investigate plasma-enhanced atomic layer deposition of cubic-phase TaCxN1−x thin films for superconducting microwave circuits. Structural and transport measurements reveal nanocrystalline morphology with sub-10 nm grains and superconductivity in the dirty limit. Coplanar waveguide resonators exhibit moderately high kinetic inductance (16.8 pH/sq for 30 nm films) with potential for enhancement through dimensional scaling. The films also support high internal quality factors exceeding 105 at 50 mK in the single-photon regime, comparable to granular aluminum. Loss analysis identifies the two-level systems as the dominant limiting mechanism, with potential for further reduction through interface engineering. These results establish atomic layer deposited TaCxN1−x as a promising material for scalable, low-loss, high-inductance superconducting circuits.

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Publication Details

Journal
Applied Physics Letters
Published
2025-11-10
DOI
https://doi.org/10.1063/5.0300902
Primary Topic
Diamond and Carbon-based Materials Research
Type
article
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article

Investigation of kinetic inductance and microwave loss in thin-film TaCxN1−x superconducting resonators

Dmytro Nykypanchuk, Xiao Tong, Sooyeon Hwang, Matthew LaHaye et al.
Applied Physics Letters
Diamond and Carbon-based Materials Research
article

Investigation of kinetic inductance and microwave loss in thin-film TaCxN1−x superconducting resonators

Dmytro Nykypanchuk, Xiao Tong, Sooyeon Hwang, Matthew LaHaye, M. D. Nguyen, Davood Shahrjerdi, Moeid Jamalzadeh, M. R. Perez, Christopher Nadeau, Iliya Shiravand
article en

Abstract

The promise of tantalum for realizing superconducting quantum devices has generated interest in its compound films, particularly nitrides. Among these, cubic-phase tantalum carbonitride (TaCxN1−x) offers reduced susceptibility to oxidation and a high critical temperature, yet its microwave properties remain largely unexplored. Here, we investigate plasma-enhanced atomic layer deposition of cubic-phase TaCxN1−x thin films for superconducting microwave circuits. Structural and transport measurements reveal nanocrystalline morphology with sub-10 nm grains and superconductivity in the dirty limit. Coplanar waveguide resonators exhibit moderately high kinetic inductance (16.8 pH/sq for 30 nm films) with potential for enhancement through dimensional scaling. The films also support high internal quality factors exceeding 105 at 50 mK in the single-photon regime, comparable to granular aluminum. Loss analysis identifies the two-level systems as the dominant limiting mechanism, with potential for further reduction through interface engineering. These results establish atomic layer deposited TaCxN1−x as a promising material for scalable, low-loss, high-inductance superconducting circuits.

Applied Physics LettersVol. 127(19)
United States Air Force Research Laboratory (US), Booz Allen Hamilton (United States) (US), State University of New York (US), Brookhaven National Laboratory (US), New York University (US)
Openalex Percentile: Top 73%
Diamond and Carbon-based Materials Research
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