Background Stability and Annual Modulation Test Using PICOLON Ultra-Pure NaI(Tl) Detector

Abstract The dark matter observation claimed by the DAMA/LIBRA experiment has been a long-standing puzzle within the particle physics community. NaI(Tl) crystals with radiopurity comparable to DAMA/LIBRA’s are essential for adequate verification. Existing experiments using a NaI(Tl) target have been hampered by the high radioactivity concentration of NaI(Tl) crystals. The Pure Inorganic Crystal Observatory for LOw-energy Neutr(al)ino (PICOLON) experiment conducts an independent search for Weakly Interacting Massive Particles using the highest-purity NaI(Tl) crystals. In 2020, a PICOLON NaI(Tl) crystal (Ingot#85) reached the same purity level as DAMA/LIBRA crystals. The DAMA/LIBRA group has stressed that verifying their signal requires high-purity NaI(Tl) crystals with long-term stability. Based on a six-month measurement, we have confirmed the long-term stability of its radiopurity. This stability provides a significant advantage for future efforts to adequately verify the DAMA/LIBRA result using NaI(Tl) crystals. In this paper, we present the background stability of purity in the Ingot#94 NaI(Tl) detector, which was produced using the Ingot#85 purification method, along with the first annual modulation search conducted by the PICOLON experiment.

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Journal
Progress of Theoretical and Experimental Physics
Published
2025-11-12
DOI
https://doi.org/10.1093/ptep/ptaf160
Primary Topic
Dark Matter and Cosmic Phenomena
Type
article
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Background Stability and Annual Modulation Test Using PICOLON Ultra-Pure NaI(Tl) Detector

K. Yasuda, K. Imagawa, S. Umehara, S. Yoshida et al.
Progress of Theoretical and Experimental Physics
Dark Matter and Cosmic Phenomena
article

Background Stability and Annual Modulation Test Using PICOLON Ultra-Pure NaI(Tl) Detector

K. Yasuda, K. Imagawa, S. Umehara, S. Yoshida, R. Hazama, K. Nakamura, T. Iida, T. Shima, Kumiko Kotera, K. Fushimi, K. Hata, A. Kozlov, Yoshio Takemoto, H. Ikeda, H. Ito, R. Orito, M. Koga, T. Kishimoto, H. Ejiri, K. Inoue, Yuto Urano
article en

Abstract

Abstract The dark matter observation claimed by the DAMA/LIBRA experiment has been a long-standing puzzle within the particle physics community. NaI(Tl) crystals with radiopurity comparable to DAMA/LIBRA’s are essential for adequate verification. Existing experiments using a NaI(Tl) target have been hampered by the high radioactivity concentration of NaI(Tl) crystals. The Pure Inorganic Crystal Observatory for LOw-energy Neutr(al)ino (PICOLON) experiment conducts an independent search for Weakly Interacting Massive Particles using the highest-purity NaI(Tl) crystals. In 2020, a PICOLON NaI(Tl) crystal (Ingot#85) reached the same purity level as DAMA/LIBRA crystals. The DAMA/LIBRA group has stressed that verifying their signal requires high-purity NaI(Tl) crystals with long-term stability. Based on a six-month measurement, we have confirmed the long-term stability of its radiopurity. This stability provides a significant advantage for future efforts to adequately verify the DAMA/LIBRA result using NaI(Tl) crystals. In this paper, we present the background stability of purity in the Ingot#94 NaI(Tl) detector, which was produced using the Ingot#85 purification method, along with the first annual modulation search conducted by the PICOLON experiment.

Progress of Theoretical and Experimental PhysicsVol. 2025(12)
Osaka Sangyo University (JP), University of Tsukuba (JP), Nakanihon Automotive College (JP), Unitika (Japan) (JP), Tohoku University (JP), Osaka Butsuryo University (JP), Toneyama National Hospital (JP), Kavli Institute for the Physics and Mathematics of the Universe (JP), Kobe University (JP), National Research Nuclear University MEPhI (RU), Tokushima University (JP), The University of Osaka (JP)
Openalex Percentile: Top 84%
Dark Matter and Cosmic Phenomena
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