Universal negative magnetoresistance in antiferromagnetic metals from symmetry breaking of electron wave functions

Layered van der Waals crystals of topologically non-trivial and trivial semimetals with antiferromagnetic (AFM) ordering of magnetic sublattice are known to exhibit a negative magnetoresistance that is well correlated with AFM magnetization changes in a magnetic field. This effect is reported in several experimental studies with EuFe2As2, EuSn2As2, EuSn2P2, etc., where the resistance decreases quadratically with field by about 5% up to the spin-polarization field. Although this effect is well documented experimentally, its theoretical explanation is missing up to date. Here, we propose a theoretical mechanism describing the observed magnetoresistance that is inherent in AFM metals and is based on violation the binary $${\hat{T}}_{2}$$ symmetry. It is almost isotropic to the field and current directions, contrary to the known mechanisms such as giant magnetoresistance and chiral anomaly. The proposed intrinsic mechanism of magnetoresistance is strong in a wide class of the layered AFM-ordered semimetals. The theoretically calculated magnetoresistance is qualitatively consistent with experimental data for crystals of various composition. Layered van der Waals crystals with antiferromagnetic ordering can exhibit magnetoresistance, as observed experimentally in several semimetals. Here, a theoretical mechanism is proposed to describe magnetoresistance in antiferromagnetic metals.

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Publication Details

Journal
Communications Materials
Published
2025-11-13
DOI
https://doi.org/10.1038/s43246-025-00970-5
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
0.00

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article

Universal negative magnetoresistance in antiferromagnetic metals from symmetry breaking of electron wave functions

A. V. Sadakov, I. R. Shein, P. D. Grigoriev, N. S. Pavlov et al.
Communications Materials
Topological Materials and Phenomena
article

Universal negative magnetoresistance in antiferromagnetic metals from symmetry breaking of electron wave functions

A. V. Sadakov, I. R. Shein, P. D. Grigoriev, N. S. Pavlov, V. M. Pudalov, I. A. Nekrasov, Е.И. Мальцев, O. A. Sobolevskiy
article en

Abstract

Layered van der Waals crystals of topologically non-trivial and trivial semimetals with antiferromagnetic (AFM) ordering of magnetic sublattice are known to exhibit a negative magnetoresistance that is well correlated with AFM magnetization changes in a magnetic field. This effect is reported in several experimental studies with EuFe2As2, EuSn2As2, EuSn2P2, etc., where the resistance decreases quadratically with field by about 5% up to the spin-polarization field. Although this effect is well documented experimentally, its theoretical explanation is missing up to date. Here, we propose a theoretical mechanism describing the observed magnetoresistance that is inherent in AFM metals and is based on violation the binary $${\hat{T}}_{2}$$ symmetry. It is almost isotropic to the field and current directions, contrary to the known mechanisms such as giant magnetoresistance and chiral anomaly. The proposed intrinsic mechanism of magnetoresistance is strong in a wide class of the layered AFM-ordered semimetals. The theoretically calculated magnetoresistance is qualitatively consistent with experimental data for crystals of various composition. Layered van der Waals crystals with antiferromagnetic ordering can exhibit magnetoresistance, as observed experimentally in several semimetals. Here, a theoretical mechanism is proposed to describe magnetoresistance in antiferromagnetic metals.

Communications MaterialsVol. 6(1)
National Research University Higher School of Economics (RU), P.N. Lebedev Physical Institute of the Russian Academy of Sciences (RU), National University of Science and Technology (RU), Landau Institute for Theoretical Physics (RU), Leibniz Institute for Solid State and Materials Research (DE), National University of Science and Technology (ZW), Complexity, Topology and Dynamics in Quantum Matter (DE), Institute of Solid State Chemistry (RU), Institute of Electrophysics (RU)
Ural Branch, Russian Academy of Sciences, Institute of Solid State Chemistry, Ural Branch, Russian Academy of Sciences
Openalex Percentile: Top 73%
Topological Materials and Phenomena
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