Terahertz Landau level spectroscopy of Dirac fermions in millimeter-scale twisted bilayer graphene

Exotic electronic physics including correlated insulating states and fractional Chern insulators have been observed in twisted bilayer graphene in a magnetic field when the Fermi velocity vanishes; however, a question remains as to the stability of these states, which is controlled by the gap to the first excited state. Free-space terahertz magneto-optics can directly probe the gap to charge excitations, which bounds the stability of electronic states, but this measurement has thus far been inaccessible due to the micron size of twisted bilayer graphene samples, while the wavelength of terahertz light is up to 1 mm. Here we leverage advances in fabrication to create twisted bilayer graphene samples over $5\ifmmode\times\else\texttimes\fi{}5$ mm in size with a uniform twist angle and study the magnetic field dependence of the cyclotron resonance by a complex Faraday rotation experiment in $p$-doped large angle twisted bilayer graphene. These measurements directly probe charge excitations in inter-Landau level transitions and determine the Fermi velocity as a function of twist angle.

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Journal
Physical review. B./Physical review. B
Published
2025-11-13
DOI
https://doi.org/10.1103/5s4k-5jtj
Primary Topic
Graphene research and applications
Type
article
Field-Weighted Citation Impact
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article

Terahertz Landau level spectroscopy of Dirac fermions in millimeter-scale twisted bilayer graphene

Debarghya Mallick, Cheol‐Joo Kim, Xingyue Han, Matthew Brahlek et al.
Physical review. B./Physical review. B
Graphene research and applications
article

Terahertz Landau level spectroscopy of Dirac fermions in millimeter-scale twisted bilayer graphene

Debarghya Mallick, Cheol‐Joo Kim, Xingyue Han, Matthew Brahlek, Spenser Talkington, E. J. Melé, Seong‐Jun Yang, Zhaodong Chu, An‐Hsi Chen, Liang Wu, Benjamin F. Mead
article en

Abstract

Exotic electronic physics including correlated insulating states and fractional Chern insulators have been observed in twisted bilayer graphene in a magnetic field when the Fermi velocity vanishes; however, a question remains as to the stability of these states, which is controlled by the gap to the first excited state. Free-space terahertz magneto-optics can directly probe the gap to charge excitations, which bounds the stability of electronic states, but this measurement has thus far been inaccessible due to the micron size of twisted bilayer graphene samples, while the wavelength of terahertz light is up to 1 mm. Here we leverage advances in fabrication to create twisted bilayer graphene samples over $5\ifmmode\times\else\texttimes\fi{}5$ mm in size with a uniform twist angle and study the magnetic field dependence of the cyclotron resonance by a complex Faraday rotation experiment in $p$-doped large angle twisted bilayer graphene. These measurements directly probe charge excitations in inter-Landau level transitions and determine the Fermi velocity as a function of twist angle.

Physical review. B./Physical review. BVol. 112(20)
Pohang University of Science and Technology (KR), Oak Ridge National Laboratory (US), California University of Pennsylvania (US), Institute for Basic Science (KR), University of Pennsylvania (US)
Openalex Percentile: Top 73%
Graphene research and applications
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