Topological metal-insulator transition within the ferromagnetic state

A major challenge in condensed matter physics is integrating topological phenomena with correlated electron physics to leverage both types of states for next-generation quantum devices. Metal-insulator transitions are central to bridging these two domains while simultaneously serving as on-off switches for electronic states. Here, we demonstrate how the prototypical material of K<sub>2</sub>Cr<sub>8</sub>O<sub>16</sub> undergoes a ferromagnetic metal-insulator transition accompanied by a change in band topology. Through inelastic x-ray and neutron scattering experiments combined with first-principles theoretical calculations, we show that this transition is not driven by a Peierls mechanism, given the lack of phonon softening. Instead, we establish the transition as a topological metal-insulator transition within the ferromagnetic phase with potential axionic properties, where electron correlations play a key role in stabilizing the insulating state. These results reveal how a metal-insulator transition provides a pathway through which magnetism, topology, and electronic correlations interact.

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Publication Details

Journal
Nature Communications
Published
2026-02-27
DOI
https://doi.org/10.1038/s41467-026-70042-w
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
0.00

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article

Topological metal-insulator transition within the ferromagnetic state

A. M. dos Santos, D. G. Mazzone, Konstantinos Papadopoulos, Martin Må̊nsson et al.
Nature Communications
Topological Materials and Phenomena
article

Topological metal-insulator transition within the ferromagnetic state

A. M. dos Santos, D. G. Mazzone, Konstantinos Papadopoulos, Martin Må̊nsson, Moritz M. Hirschmann, J. Chang, Deepak John Mukkattukavil, Jun Sugiyama, Nami Matsubara, N. Gauthier, Chin Shen Ong, Masahiko Isobe, Olle Eriksson, Masafumi Horio, Hiroshi Uchiyama, Ola Kenji Forslund, Christian Tzschaschel, Kazuya Kamazawa, Yasmine Sassa, Romain Sibille, Hidenori Takagi, Kazuhiko Ikeuchi, Elisabetta Nocerino
article en

Abstract

A major challenge in condensed matter physics is integrating topological phenomena with correlated electron physics to leverage both types of states for next-generation quantum devices. Metal-insulator transitions are central to bridging these two domains while simultaneously serving as on-off switches for electronic states. Here, we demonstrate how the prototypical material of K<sub>2</sub>Cr<sub>8</sub>O<sub>16</sub> undergoes a ferromagnetic metal-insulator transition accompanied by a change in band topology. Through inelastic x-ray and neutron scattering experiments combined with first-principles theoretical calculations, we show that this transition is not driven by a Peierls mechanism, given the lack of phonon softening. Instead, we establish the transition as a topological metal-insulator transition within the ferromagnetic phase with potential axionic properties, where electron correlations play a key role in stabilizing the insulating state. These results reveal how a metal-insulator transition provides a pathway through which magnetism, topology, and electronic correlations interact.

Nature CommunicationsVol. 17(1)
Uppsala University (SE), Oak Ridge National Laboratory (US), High Energy Accelerator Research Organization (JP), Stockholm University (SE), University of Zurich (CH), Institut National de la Recherche Scientifique (CA), Max Planck Institute for Solid State Research (DE), SPring-8 (JP), Japan Synchrotron Radiation Research Institute (JP), RIKEN Center for Emergent Matter Science (JP), Comprehensive Research Organization for Science and Society (JP), Chalmers University of Technology (SE), KTH Royal Institute of Technology (SE)
U.S. Department of Energy, Deutsche Forschungsgemeinschaft, Stiftelsen för Strategisk Forskning, Knut och Alice Wallenbergs Stiftelse, Paul Scherrer Institut, Vetenskapsrådet, Uppsala Universitet, Office of Science, Japan Society for the Promotion of Science, RIKEN, Oak Ridge National Laboratory
Openalex Percentile: Top 98%
Topological Materials and Phenomena
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