A Heuristic Time-Domain Raman Forward Solver for Photon Migration in a Two-Layer Diffusive Medium

An analytical heuristic model has been developed to describe the time-domain reflectance Raman signal in a two-layer diffusive medium. The model is based on the solution of two coupled diffusion equations at the excitation and emission wavelengths, respectively. The accuracy of the model is verified by comparison with the results of Monte Carlo simulations. This solver correctly accounts for the Raman emitters within the layers and the full wavelength dependence of the optical properties of the layers. The computational efficiency of the solver is compatible with the requirements of rapid reconstructions of Raman spectra from time-domain Raman measurements acquired for a large number of different wavelengths.

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Publication Details

Journal
Photonics
Published
2025-11-11
DOI
https://doi.org/10.3390/photonics12111114
Primary Topic
Optical Imaging and Spectroscopy Techniques
Type
article
Field-Weighted Citation Impact
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article

A Heuristic Time-Domain Raman Forward Solver for Photon Migration in a Two-Layer Diffusive Medium

Alessandro Bossi, Fabrizio Martelli, Antonio Pifferi, Stefan Šušnjar et al.
Photonics
Optical Imaging and Spectroscopy Techniques
article

A Heuristic Time-Domain Raman Forward Solver for Photon Migration in a Two-Layer Diffusive Medium

Alessandro Bossi, Fabrizio Martelli, Antonio Pifferi, Stefan Šušnjar, Federico Tommasi, Andrea Farina, Ilaria Bargigia, Naseer Kammalamuriyil
article en

Abstract

An analytical heuristic model has been developed to describe the time-domain reflectance Raman signal in a two-layer diffusive medium. The model is based on the solution of two coupled diffusion equations at the excitation and emission wavelengths, respectively. The accuracy of the model is verified by comparison with the results of Monte Carlo simulations. This solver correctly accounts for the Raman emitters within the layers and the full wavelength dependence of the optical properties of the layers. The computational efficiency of the solver is compatible with the requirements of rapid reconstructions of Raman spectra from time-domain Raman measurements acquired for a large number of different wavelengths.

PhotonicsVol. 12(11)
Istituto Nazionale di Fisica Nucleare, Sezione di Firenze (IT), Istituto di Fotonica e Nanotecnologie (IT), SpectraCure (Sweden) (SE), University of Florence (IT), Politecnico di Milano (IT)
Openalex Percentile: Top 51%
Optical Imaging and Spectroscopy Techniques
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A Heuristic Time-Domain Raman Forward Solver for Photon Migration in a Two-Layer Diffusive Medium — Alessandro Bossi, Fabrizio Martelli, et al. · Photonics (2025) | TGRS Research Map | TGRS