Characterization of Complex Stacking of Semiconductors Through Near Field Imaging and Spectroscopy

While high operating temperature infrared photodetection remains a major technological objective, huge improvements have been obtained through the use of increasingly complex semiconductors epitaxies such as quantum cascade structures or III-V superlattice junction. However, the characterization of these layers is challenging and often requires the use of destructive processes. Here, SNOM imaging and spectroscopy on a mechanically cleaved facet is used to characterize the different layers of a complex epitaxial heterostructure composed of a type II superlattice and highly doped semiconductors. These near-field experimental data are compared to simulation in order to retrieve both the cut-off frequency of the superlattice and the doping level of each highly doped semiconductor layers. Additionally, information about interfaces is optically retrieved through hyperspectral characterization of plasmons propagating at these vertical interfaces. In parallel, all the materials and exact stacking of the epitaxy are confirmed through scanning transmission electron microscopy.

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Publication Details

Journal
Advanced Materials
Published
2025-11-10
DOI
https://doi.org/10.1002/adma.202507645
Primary Topic
Near-Field Optical Microscopy
Type
article
Field-Weighted Citation Impact
0.00

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article

Characterization of Complex Stacking of Semiconductors Through Near Field Imaging and Spectroscopy

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Advanced Materials
Near-Field Optical Microscopy
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Characterization of Complex Stacking of Semiconductors Through Near Field Imaging and Spectroscopy

Jean‐Baptiste Rodriguez, Baptiste Fix, Frédéric Fossard, Jean‐Sébastien Mérot, Grégory Vincent, T. Taliercio, F. González‐Posada, Clément Gureghian, Laure Tailpied
article en

Abstract

While high operating temperature infrared photodetection remains a major technological objective, huge improvements have been obtained through the use of increasingly complex semiconductors epitaxies such as quantum cascade structures or III-V superlattice junction. However, the characterization of these layers is challenging and often requires the use of destructive processes. Here, SNOM imaging and spectroscopy on a mechanically cleaved facet is used to characterize the different layers of a complex epitaxial heterostructure composed of a type II superlattice and highly doped semiconductors. These near-field experimental data are compared to simulation in order to retrieve both the cut-off frequency of the superlattice and the doping level of each highly doped semiconductor layers. Additionally, information about interfaces is optically retrieved through hyperspectral characterization of plasmons propagating at these vertical interfaces. In parallel, all the materials and exact stacking of the epitaxy are confirmed through scanning transmission electron microscopy.

Advanced MaterialsVol. 38(7)
Centre National de la Recherche Scientifique (FR), Université Paris-Saclay (FR), Sorbonne Université (FR), Centre Inria de Saclay (FR), Laboratoire d'Étude des Microstructures (FR), Institut d'Électronique et des Systèmes (FR), Institut des NanoSciences de Paris (FR)
Equipex, Agence Nationale de la Recherche, Agence de l'innovation de Défense
Openalex Percentile: Top 67%
Near-Field Optical Microscopy
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