Interface density driven metal-to-insulator transition in nickelate based heterostructures

Heterostructures made of alternating metallic layers of <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi>Nd</a:mi> <a:mrow> <a:mn>0.7</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi>La</a:mi> <a:mrow> <a:mn>0.3</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi>NiO</a:mi> <a:mn>3</a:mn> </a:msub> </a:mrow> </a:math> and layers displaying a metal-to-insulator transition (such as <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:msub> <b:mi>SmNiO</b:mi> <b:mn>3</b:mn> </b:msub> </b:math> ) have been grown varying the period of the superlattices on top of <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:msub> <c:mi>LaAlO</c:mi> <c:mn>3</c:mn> </c:msub> </c:math> substrates. Exploiting the phase boundary cost found between metallic and insulating phases of nickelates, it is shown that a metallic layer can be turned into an insulating one by means of heterostructuring in an intermediate thickness regime in which the single layers retain their metallic behavior.

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Journal
Physical Review Materials
Published
2025-11-10
DOI
https://doi.org/10.1103/syz5-9cbc
Primary Topic
Magnetic and transport properties of perovskites and related materials
Type
article
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article

Interface density driven metal-to-insulator transition in nickelate based heterostructures

Chih‐Ying Hsu, Lucia Varbaro, Alexandru Bogdan Georgescu, Jean‐Marc Triscone et al.
Physical Review Materials
Magnetic and transport properties of perovskites and related materials
article

Interface density driven metal-to-insulator transition in nickelate based heterostructures

Chih‐Ying Hsu, Lucia Varbaro, Alexandru Bogdan Georgescu, Jean‐Marc Triscone, Lukas Korosec, Duncan T. L. Alexander
article en

Abstract

Heterostructures made of alternating metallic layers of <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi>Nd</a:mi> <a:mrow> <a:mn>0.7</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi>La</a:mi> <a:mrow> <a:mn>0.3</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi>NiO</a:mi> <a:mn>3</a:mn> </a:msub> </a:mrow> </a:math> and layers displaying a metal-to-insulator transition (such as <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:msub> <b:mi>SmNiO</b:mi> <b:mn>3</b:mn> </b:msub> </b:math> ) have been grown varying the period of the superlattices on top of <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:msub> <c:mi>LaAlO</c:mi> <c:mn>3</c:mn> </c:msub> </c:math> substrates. Exploiting the phase boundary cost found between metallic and insulating phases of nickelates, it is shown that a metallic layer can be turned into an insulating one by means of heterostructuring in an intermediate thickness regime in which the single layers retain their metallic behavior.

Physical Review MaterialsVol. 9(11)
University of Geneva (CH), Indiana University Bloomington (US), École Polytechnique Fédérale de Lausanne (CH), Indiana University (US)
Openalex Percentile: Top 76%
Magnetic and transport properties of perovskites and related materials
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Interface density driven metal-to-insulator transition in nickelate based heterostructures — Chih‐Ying Hsu, Lucia Varbaro, et al. · Physical Review Materials (2025) | TGRS Research Map | TGRS