Interface density driven metal-to-insulator transition in nickelate based heterostructures
Heterostructures made of alternating metallic layers of <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi>Nd</a:mi> <a:mrow> <a:mn>0.7</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi>La</a:mi> <a:mrow> <a:mn>0.3</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi>NiO</a:mi> <a:mn>3</a:mn> </a:msub> </a:mrow> </a:math> and layers displaying a metal-to-insulator transition (such as <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:msub> <b:mi>SmNiO</b:mi> <b:mn>3</b:mn> </b:msub> </b:math> ) have been grown varying the period of the superlattices on top of <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:msub> <c:mi>LaAlO</c:mi> <c:mn>3</c:mn> </c:msub> </c:math> substrates. Exploiting the phase boundary cost found between metallic and insulating phases of nickelates, it is shown that a metallic layer can be turned into an insulating one by means of heterostructuring in an intermediate thickness regime in which the single layers retain their metallic behavior.
Authors
- Chih‐Ying Hsu (ORCID: https://orcid.org/0000-0001-7141-3046)
- Lucia Varbaro (ORCID: https://orcid.org/0000-0001-7128-7174)
- Alexandru Bogdan Georgescu (ORCID: https://orcid.org/0000-0002-3161-1491)
- Jean‐Marc Triscone (ORCID: https://orcid.org/0000-0002-9067-701X)
- Lukas Korosec (ORCID: https://orcid.org/0000-0003-4962-7923)
- Duncan T. L. Alexander (ORCID: https://orcid.org/0000-0003-4350-8587)
Institutions
- University of Geneva (CH)
- Indiana University Bloomington (US)
- École Polytechnique Fédérale de Lausanne (CH)
- Indiana University (US)
Publication Details
- Journal
- Physical Review Materials
- Published
- 2025-11-10
- DOI
- https://doi.org/10.1103/syz5-9cbc
- Primary Topic
- Magnetic and transport properties of perovskites and related materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00