Infrared Photothermal Heterodyne Imaging in Thermally Thick Medium for Thermo-optic Property Characterizations

Measuring temperature fields in semitransparent media requires the knowledge of material thermo-optic properties. While the current techniques are well established for isothermal thin films, they remain unexplored for thick media where temperature gradients need to be considered. This study proposes to generalize the current methods of infrared heterodyne photothermal imaging to thick media by combining transmittance measurements and thermo-optic modeling to measure simultaneously the thermoabsorbance and thermoreflectance coefficients in semitransparent material. In this work, we demonstrate the validity of our methodology followed by the measurements of the thermo-optic properties of several materials: soft polymers (polydimethylsiloxane) and borofloat glasses.

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Publication Details

Journal
The Journal of Physical Chemistry Letters
Published
2025-11-10
DOI
https://doi.org/10.1021/acs.jpclett.5c01503
Primary Topic
Thermography and Photoacoustic Techniques
Type
article
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article

Infrared Photothermal Heterodyne Imaging in Thermally Thick Medium for Thermo-optic Property Characterizations

Jérémie Maire, Stéphane Chevalier, A Netter, Jordan Letessier
The Journal of Physical Chemistry Letters
Thermography and Photoacoustic Techniques
article

Infrared Photothermal Heterodyne Imaging in Thermally Thick Medium for Thermo-optic Property Characterizations

Jérémie Maire, Stéphane Chevalier, A Netter, Jordan Letessier
article en

Abstract

Measuring temperature fields in semitransparent media requires the knowledge of material thermo-optic properties. While the current techniques are well established for isothermal thin films, they remain unexplored for thick media where temperature gradients need to be considered. This study proposes to generalize the current methods of infrared heterodyne photothermal imaging to thick media by combining transmittance measurements and thermo-optic modeling to measure simultaneously the thermoabsorbance and thermoreflectance coefficients in semitransparent material. In this work, we demonstrate the validity of our methodology followed by the measurements of the thermo-optic properties of several materials: soft polymers (polydimethylsiloxane) and borofloat glasses.

The Journal of Physical Chemistry LettersVol. 16(46)
Centre National de la Recherche Scientifique (FR), Université de Bordeaux (FR), Arts et Métiers (FR), Institut de Mécanique et d'Ingénierie de Bordeaux (FR), Institut Polytechnique de Bordeaux (FR), The University of Tokyo (JP)
Openalex Percentile: Top 62%
Thermography and Photoacoustic Techniques
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