Anomalous Nodal Gap in a Doped Spin- <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mn>1</mml:mn> <mml:mo>/</mml:mo> <mml:mn>2</mml:mn> </mml:mrow> </mml:math> Antiferromagnetic Mott Insulator

Many emergent phenomena appear in doped Mott insulators near the insulator-to-metal transition. In high-temperature cuprate superconductors, superconductivity arises when antiferromagnetic (AFM) order is gradually suppressed by carrier doping, and a d-wave superconducting gap forms when an enigmatic nodal gap evolves into a point node. Here, we examine electron-doped Sr_{2}IrO_{4}, the 5d-electron counterpart of cuprates, using angle-resolved photoemission spectroscopy. At low doping levels, we observe the formation of electronic states near the Fermi level, accompanied by a gap at the AFM zone boundary, mimicking the AFM gap in electron-doped cuprates. With increasing doping, a distinct gap emerges along the (0,0)-(π,π) nodal direction, paralleling that observed in hole-doped cuprates. This anomalous nodal gap persists after the collapse of the AFM gap and gradually decreases with further doping. It eventually vanishes into a point node of the reported d-wave gap. These observations replicate the characteristic features in both electron- and hole-doped cuprates, indicating a unified route toward nodal metallicity in doped spin-1/2 AFM Mott insulators.

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Publication Details

Journal
Physical Review Letters
Published
2025-11-07
DOI
https://doi.org/10.1103/3rw4-mhz8
Primary Topic
Physics of Superconductivity and Magnetism
Type
article
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article

Anomalous Nodal Gap in a Doped Spin- <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mn>1</mml:mn> <mml:mo>/</mml:mo> <mml:mn>2</mml:mn> </mml:mrow> </mml:math> Antiferromagnetic Mott Insulator

Jun-Feng He, Stephen D. Wilson, Yong Hu, Arun Bansil et al.
Physical Review Letters
Physics of Superconductivity and Magnetism
article

Anomalous Nodal Gap in a Doped Spin- <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mn>1</mml:mn> <mml:mo>/</mml:mo> <mml:mn>2</mml:mn> </mml:mrow> </mml:math> Antiferromagnetic Mott Insulator

Jun-Feng He, Stephen D. Wilson, Yong Hu, Arun Bansil, Dong-Hui Lu, Tao Wu, R. S. Markiewicz, Makoto Hashimoto, Shuting Peng, Christopher Lane, Xiang Chen, Zeliang Sun, Xianhui Chen
article en

Abstract

Many emergent phenomena appear in doped Mott insulators near the insulator-to-metal transition. In high-temperature cuprate superconductors, superconductivity arises when antiferromagnetic (AFM) order is gradually suppressed by carrier doping, and a d-wave superconducting gap forms when an enigmatic nodal gap evolves into a point node. Here, we examine electron-doped Sr_{2}IrO_{4}, the 5d-electron counterpart of cuprates, using angle-resolved photoemission spectroscopy. At low doping levels, we observe the formation of electronic states near the Fermi level, accompanied by a gap at the AFM zone boundary, mimicking the AFM gap in electron-doped cuprates. With increasing doping, a distinct gap emerges along the (0,0)-(π,π) nodal direction, paralleling that observed in hole-doped cuprates. This anomalous nodal gap persists after the collapse of the AFM gap and gradually decreases with further doping. It eventually vanishes into a point node of the reported d-wave gap. These observations replicate the characteristic features in both electron- and hole-doped cuprates, indicating a unified route toward nodal metallicity in doped spin-1/2 AFM Mott insulators.

Physical Review LettersVol. 135(19)
University of Science and Technology of China (CN), Northeastern University (US), Los Alamos National Laboratory (US), University of California, Santa Barbara (US), Chongqing University (CN), SLAC National Accelerator Laboratory (US), University of California System (US), Stanford Synchrotron Radiation Lightsource (US), Center for Integrated Nanotechnologies (US), Universidad del Noreste (MX)
Openalex Percentile: Top 79%
Physics of Superconductivity and Magnetism
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