Anomalous Nodal Gap in a Doped Spin- <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:mn>1</mml:mn> <mml:mo>/</mml:mo> <mml:mn>2</mml:mn> </mml:mrow> </mml:math> Antiferromagnetic Mott Insulator
Many emergent phenomena appear in doped Mott insulators near the insulator-to-metal transition. In high-temperature cuprate superconductors, superconductivity arises when antiferromagnetic (AFM) order is gradually suppressed by carrier doping, and a d-wave superconducting gap forms when an enigmatic nodal gap evolves into a point node. Here, we examine electron-doped Sr_{2}IrO_{4}, the 5d-electron counterpart of cuprates, using angle-resolved photoemission spectroscopy. At low doping levels, we observe the formation of electronic states near the Fermi level, accompanied by a gap at the AFM zone boundary, mimicking the AFM gap in electron-doped cuprates. With increasing doping, a distinct gap emerges along the (0,0)-(π,π) nodal direction, paralleling that observed in hole-doped cuprates. This anomalous nodal gap persists after the collapse of the AFM gap and gradually decreases with further doping. It eventually vanishes into a point node of the reported d-wave gap. These observations replicate the characteristic features in both electron- and hole-doped cuprates, indicating a unified route toward nodal metallicity in doped spin-1/2 AFM Mott insulators.
Authors
- Jun-Feng He (ORCID: https://orcid.org/0000-0001-5584-9827)
- Stephen D. Wilson (ORCID: https://orcid.org/0000-0003-3733-930X)
- Yong Hu (ORCID: https://orcid.org/0000-0002-4997-4143)
- Arun Bansil (ORCID: https://orcid.org/0000-0002-3864-3461)
- Dong-Hui Lu (ORCID: https://orcid.org/0000-0002-9708-0443)
- Tao Wu (ORCID: https://orcid.org/0000-0001-9805-4434)
- R. S. Markiewicz (ORCID: https://orcid.org/0000-0002-0747-0713)
- Makoto Hashimoto (ORCID: https://orcid.org/0000-0003-1689-8997)
- Shuting Peng (ORCID: https://orcid.org/0000-0001-7967-2288)
- Christopher Lane (ORCID: https://orcid.org/0000-0003-2945-9352)
- Xiang Chen (ORCID: https://orcid.org/0000-0003-3997-8148)
- Zeliang Sun
- Xianhui Chen
Institutions
- University of Science and Technology of China (CN)
- Northeastern University (US)
- Los Alamos National Laboratory (US)
- University of California, Santa Barbara (US)
- Chongqing University (CN)
- SLAC National Accelerator Laboratory (US)
- University of California System (US)
- Stanford Synchrotron Radiation Lightsource (US)
- Center for Integrated Nanotechnologies (US)
- Universidad del Noreste (MX)
Publication Details
- Journal
- Physical Review Letters
- Published
- 2025-11-07
- DOI
- https://doi.org/10.1103/3rw4-mhz8
- Primary Topic
- Physics of Superconductivity and Magnetism
- Type
- article
- Field-Weighted Citation Impact
- 0.00