Broadband high-resolution X-ray ptychography system spanning tender to hard X-ray regimes
X-ray ptychography is a high-resolution imaging technique capable of resolving nanoscale structures and probing chemical states. However, despite advances, most conventional X-ray ptychography systems have been designed to operate within a single energy regime, such as hard (> 5 keV), soft (< 2 keV) or tender (2-5 keV) X-rays. We have developed a high-efficiency achromatic ptychographic measurement system on beamline BL10U at NanoTerasu, a 3 GeV synchrotron radiation facility in Japan, that incorporates advanced Kirkpatrick-Baez focusing mirrors and a high-speed CITIUS detector. Utilizing this innovative system, we have successfully reconstructed phase images with a spatial resolution exceeding 50 nm from 200 nm-thick tantalum test charts at X-ray energies of 2.5, 5.0 and 7.5 keV. We have performed energy scans around the Ca and S K edges on CaSO<sub>4</sub>·2H<sub>2</sub>O particles to demonstrate the spectromicroscopic capabilities of the system. The reconstructed images provide spatially resolved X-ray absorption spectra, revealing distinct edge features. This system not only enables element-specific imaging across the tender to hard X-ray spectrum but is also particularly advantageous for light-element materials, which benefit from enhanced phase contrast in the tender X-ray range. This advancement opens up new possibilities for in situ imaging of complex chemical environments in energy devices and biological specimens.
Authors
- Fusae Kaneko
- Hideshi Uematsu
- Shuntaro Takazawa
- Nozomu Ishiguro (ORCID: https://orcid.org/0000-0003-3330-6236)
- Yukio Takahashi (ORCID: https://orcid.org/0000-0001-8506-4289)
- Masaki Abe (ORCID: https://orcid.org/0009-0002-1369-629X)
- Yuhei Sasaki
- Naru Okawa
Institutions
- Tohoku University (JP)
Publication Details
- Journal
- IUCrJ
- Published
- 2025-11-06
- DOI
- https://doi.org/10.1107/s2052252525009236
- Primary Topic
- Advanced X-ray Imaging Techniques
- Type
- article
- Field-Weighted Citation Impact
- 0.00