Uneven Co–N–C-coated graphene as a durable support for low-loading Pt oxygen reduction catalyst

An uneven Co-N-C layer coated on electrochemically-exfoliated graphene as an active support (<i>E</i><sub>1/2</sub> 0.788 V) to stabilize low-amount Pt catalyst was synthesized. The catalyst exhibited superior oxygen reduction activity (0.72 A mg<sub>Pt</sub><sup>-1</sup>) and durability (10 mV loss after 50k cycles) in acid. Graphene reinforced the metal-support interaction, benefitting the conductivity, activity and durability of the catalyst.

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Publication Details

Journal
Chemical Communications
Published
2025-01-01
DOI
https://doi.org/10.1039/d5cc05415j
Primary Topic
Electrocatalysts for Energy Conversion
Type
article
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article

Uneven Co–N–C-coated graphene as a durable support for low-loading Pt oxygen reduction catalyst

Junzhong Wang, Junying Wang, Zelin Wu, Huinian Zhang et al.
Chemical Communications
Electrocatalysts for Energy Conversion
article

Uneven Co–N–C-coated graphene as a durable support for low-loading Pt oxygen reduction catalyst

Junzhong Wang, Junying Wang, Zelin Wu, Huinian Zhang, Ruoxuan Zhi, Jun Wang, Ming Xu, Yichen Wei, Wenhui Ni, Mingyu Liu
article en

Abstract

An uneven Co-N-C layer coated on electrochemically-exfoliated graphene as an active support (<i>E</i><sub>1/2</sub> 0.788 V) to stabilize low-amount Pt catalyst was synthesized. The catalyst exhibited superior oxygen reduction activity (0.72 A mg<sub>Pt</sub><sup>-1</sup>) and durability (10 mV loss after 50k cycles) in acid. Graphene reinforced the metal-support interaction, benefitting the conductivity, activity and durability of the catalyst.

Chemical CommunicationsVol. 61(96)
North University of China (CN), Anhui University (CN), Chinese Academy of Sciences (CN), Institute of Coal Chemistry (CN)
Openalex Percentile: Top 77%
Electrocatalysts for Energy Conversion
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Uneven Co–N–C-coated graphene as a durable support for low-loading Pt oxygen reduction catalyst — Junzhong Wang, Junying Wang, et al. · Chemical Communications (2025) | TGRS Research Map | TGRS