Emulating chemistry-climate dynamics with a linear inverse model

Abstract. Coupled chemistry–climate models (CCMs) are powerful tools for investigating chemical variability in the climate system, but high computational cost limits their use for hypothesis testing and adequately sampling variability on long timescales. Here, we present the first application of a linear inverse model (LIM) to emulate a CCM. A LIM is a low-dimensional empirical model that reproduces the CCM's statistics and dynamics at low computational cost. By linearizing the CCM's dynamics, the LIM captures coherent modes of variability, such as the El Niño Southern Oscillation (ENSO), that describe the coupled evolution of physical and chemical fields. Deterministic seasonal forecasts of the LIM result in skillful predictions of physical and chemical variables at lead times up to a year, outperforming damped persistence models. We show that the LIM's skill in chemical fields depends on its coupled chemistry–climate modes: forecasts without the ENSO dynamical mode show a substantial loss of skill, suggesting the importance of ENSO in driving predictable chemical variability. These results demonstrate that the LIM can efficiently emulate CCM dynamics. It offers a practical tool for testing hypotheses about the drivers of chemistry-climate interactions and may enable efficient chemical data assimilation in the future.

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Publication Details

Journal
Atmospheric chemistry and physics
Published
2025-11-07
DOI
https://doi.org/10.5194/acp-25-15033-2025
Primary Topic
Climate variability and models
Type
article
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article

Emulating chemistry-climate dynamics with a linear inverse model

Alexander Jay Turner, Gregory J. Hakim, Eric J. Mei, Max Taniguchi-King et al.
Atmospheric chemistry and physics
Climate variability and models
article

Emulating chemistry-climate dynamics with a linear inverse model

Alexander Jay Turner, Gregory J. Hakim, Eric J. Mei, Max Taniguchi-King, Dominik Stiller
article en

Abstract

Abstract. Coupled chemistry–climate models (CCMs) are powerful tools for investigating chemical variability in the climate system, but high computational cost limits their use for hypothesis testing and adequately sampling variability on long timescales. Here, we present the first application of a linear inverse model (LIM) to emulate a CCM. A LIM is a low-dimensional empirical model that reproduces the CCM's statistics and dynamics at low computational cost. By linearizing the CCM's dynamics, the LIM captures coherent modes of variability, such as the El Niño Southern Oscillation (ENSO), that describe the coupled evolution of physical and chemical fields. Deterministic seasonal forecasts of the LIM result in skillful predictions of physical and chemical variables at lead times up to a year, outperforming damped persistence models. We show that the LIM's skill in chemical fields depends on its coupled chemistry–climate modes: forecasts without the ENSO dynamical mode show a substantial loss of skill, suggesting the importance of ENSO in driving predictable chemical variability. These results demonstrate that the LIM can efficiently emulate CCM dynamics. It offers a practical tool for testing hypotheses about the drivers of chemistry-climate interactions and may enable efficient chemical data assimilation in the future.

Atmospheric chemistry and physicsVol. 25(21)
Planetary Science Institute (US), University of Washington (US), University of California, Berkeley (US)
Openalex Percentile: Top 69%
Climate variability and models
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Emulating chemistry-climate dynamics with a linear inverse model — Alexander Jay Turner, Gregory J. Hakim, et al. · Atmospheric chemistry and physics (2025) | TGRS Research Map | TGRS