Lightwave control of many-body interaction-driven petahertz photocurrent
Light-field-driven currents sensitive to pulse waveforms have established a promising foundation for the realization of petahertz (PHz) electronic devices. However, the influence of many-body interactions on photocurrent generation remains inadequately understood. Here, we theoretically investigate photocurrent generation in monolayer $\mathrm{Mo}{\mathrm{S}}_{2}$, highlighting the essential role of many-body effect on carrier dynamics and the optoelectronic response. We demonstrate that photocurrents depend critically on the electric-field waveform controlled by the carrier-envelope phase, and we reveal a distinct signature of multielectron interactions manifested as destructive interference of the maximum current with increasing field strength, due to specific intraband Coulomb scattering processes that can induce a primary band energy renormalization. Additionally, we propose an optical switch based on two orthogonally linearly polarized laser pulses with a controlled delay, capable of achieving current modulation at frequencies approaching 1 PHz. We present a strategy for constructing logic gates and emphasize the critical role of many-body interactions in the implementation of their functionality encoding. This optical switch also provides an all-electronic method to measure dephasing time on femtosecond timescales. Our findings deepen the understanding of many-body effects in petahertz electronics and facilitate the development of ultrafast optoelectronic devices based on two-dimensional materials.
Authors
- Candong Liu (ORCID: https://orcid.org/0000-0001-9319-3080)
- Ya Bai (ORCID: https://orcid.org/0000-0003-3953-0001)
- Yu Chen (ORCID: https://orcid.org/0000-0003-3058-1240)
- Ruxin Li
- Ying Ma (ORCID: https://orcid.org/0000-0001-6473-4044)
Institutions
- Tongji University (CN)
- Shanghai Zhangjiang Laboratory (CN)
- Shanghai Institute of Optics and Fine Mechanics (CN)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-11-06
- DOI
- https://doi.org/10.1103/4fcn-rq3r
- Citations
- 1
- Primary Topic
- Terahertz technology and applications
- Type
- article
- Field-Weighted Citation Impact
- 0.73