Photoinduced melting dynamics and collective mode in a correlated charge-ordered system

We theoretically investigate the transient spectral function during the photoinduced melting of charge order in a correlated electron system, to unravel the dynamical processes triggered by different initial excitations. We employ a one-dimensional interacting spinless fermion model introducing a pulsed laser light, and perform a comparative study by the Hartree-Fock approximation and by the exact diagonalization method to numerically solve the time-dependent Schrödinger equation. We find characteristic behavior in the transient spectral function, whose features strongly depend on the pump light frequency $ω_p$. When $ω_p$ is resonant with the collective phase mode of frequency $Ω_c\simeq Δ_{\rm CO}/2$, where $Δ_{\rm CO}$ is the charge gap, the transient spectral function exhibits a photoinduced in-gap weight which triggers large responses. With increasing the laser intensity, the development of in-gap weight directly turns into the collapse of the gap. This charge-order destabilization process is in sharp contrast to the case of $ω_p>Δ_{\rm CO}$, where the photoirradiation induces interband electron-hole excitations giving rise to a shrinkage of the gap. The impact of quantum fluctuations and spatial inhomogeneity on the photoinduced dynamics is also discussed.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2026-02-23
DOI
https://doi.org/10.1103/mz8w-3vgz
Primary Topic
Quantum and electron transport phenomena
Type
article
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article

Photoinduced melting dynamics and collective mode in a correlated charge-ordered system

Hitoshi Seo, Yasuhiro Tanaka
Physical review. B./Physical review. B
Quantum and electron transport phenomena
article

Photoinduced melting dynamics and collective mode in a correlated charge-ordered system

Hitoshi Seo, Yasuhiro Tanaka
article en

Abstract

We theoretically investigate the transient spectral function during the photoinduced melting of charge order in a correlated electron system, to unravel the dynamical processes triggered by different initial excitations. We employ a one-dimensional interacting spinless fermion model introducing a pulsed laser light, and perform a comparative study by the Hartree-Fock approximation and by the exact diagonalization method to numerically solve the time-dependent Schrödinger equation. We find characteristic behavior in the transient spectral function, whose features strongly depend on the pump light frequency $ω_p$. When $ω_p$ is resonant with the collective phase mode of frequency $Ω_c\simeq Δ_{\rm CO}/2$, where $Δ_{\rm CO}$ is the charge gap, the transient spectral function exhibits a photoinduced in-gap weight which triggers large responses. With increasing the laser intensity, the development of in-gap weight directly turns into the collapse of the gap. This charge-order destabilization process is in sharp contrast to the case of $ω_p>Δ_{\rm CO}$, where the photoirradiation induces interband electron-hole excitations giving rise to a shrinkage of the gap. The impact of quantum fluctuations and spatial inhomogeneity on the photoinduced dynamics is also discussed.

Physical review. B./Physical review. BVol. 113(12)
Kanazawa Institute of Technology (JP), RIKEN Center for Emergent Matter Science (JP)
Openalex Percentile: Top 99%
Quantum and electron transport phenomena
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