Photoinduced excitonic magnetism in a multiorbital Hubbard system

Multiorbital Hubbard models with Hund coupling and crystal-field splitting exhibit an instability toward spin-triplet excitonic order in the parameter regime characterized by strong local spin fluctuations. Upon chemical doping, two distinct types of excitonic ferromagnetism have been reported. Using steady-state nonequilibrium dynamical mean-field theory, we demonstrate that photo-doped half-filled systems can host nonthermal counterparts of these excitonic phases and exhibit a rich phase diagram in the space of photo-doping and crystal field splitting. Photo-doping a spin-triplet excitonic insulator provides a route towards nonequilibrium control of magnetic order.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2026-01-05
DOI
https://doi.org/10.1103/x12m-1s8v
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
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article

Photoinduced excitonic magnetism in a multiorbital Hubbard system

Sujay Ray, Lei Geng, Philipp Werner
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
article

Photoinduced excitonic magnetism in a multiorbital Hubbard system

Sujay Ray, Lei Geng, Philipp Werner
article en

Abstract

Multiorbital Hubbard models with Hund coupling and crystal-field splitting exhibit an instability toward spin-triplet excitonic order in the parameter regime characterized by strong local spin fluctuations. Upon chemical doping, two distinct types of excitonic ferromagnetism have been reported. Using steady-state nonequilibrium dynamical mean-field theory, we demonstrate that photo-doped half-filled systems can host nonthermal counterparts of these excitonic phases and exhibit a rich phase diagram in the space of photo-doping and crystal field splitting. Photo-doping a spin-triplet excitonic insulator provides a route towards nonequilibrium control of magnetic order.

Physical review. B./Physical review. BVol. 113(3)
University of Fribourg (CH)
Openalex Percentile: Top 99%
Advanced Condensed Matter Physics
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