Demonstration of Miexciton: enhancement of light–matter interaction in monolayer WS <sub>2</sub> on a Si metasurface

Two-dimensional transition metal dichalcogenides (TMDCs) semiconductors are promising for photonic and optoelectronic applications, but their atomic thickness limits photon harvesting. Here, we demonstrate the Miexciton hybrid states arising from intermediate coherent coupling between monolayer WS<sub>2</sub> excitons and Mie resonances in a dielectric Huygens silicon metasurface. Spectroscopic measurements show a Rabi splitting of ~81 meV, closely matching simulations, corresponding to WS<sub>2</sub> absorption exceeding 0.62. Photoluminescence reveals an 18-fold enhancement in emission intensity relative to WS<sub>2</sub> on quartz, driven by strong near-field confinement and an increased optical density of states. This approach provides a robust pathway to boost excitonic absorption and emission, advancing integrated optoelectronic platforms based on atomically thin crystals.

Authors

Publication Details

Journal
Optics Letters
Published
2025-11-05
DOI
https://doi.org/10.1364/ol.579124
Citations
1
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.52
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article

Demonstration of Miexciton: enhancement of light–matter interaction in monolayer WS 2 on a Si metasurface

Junichi Takahara, Dingwei Chen
1 citations
Optics Letters
2D Materials and Applications
0.52
article

Demonstration of Miexciton: enhancement of light–matter interaction in monolayer WS 2 on a Si metasurface

Junichi Takahara, Dingwei Chen
article en
1 citations

Abstract

Two-dimensional transition metal dichalcogenides (TMDCs) semiconductors are promising for photonic and optoelectronic applications, but their atomic thickness limits photon harvesting. Here, we demonstrate the Miexciton hybrid states arising from intermediate coherent coupling between monolayer WS<sub>2</sub> excitons and Mie resonances in a dielectric Huygens silicon metasurface. Spectroscopic measurements show a Rabi splitting of ~81 meV, closely matching simulations, corresponding to WS<sub>2</sub> absorption exceeding 0.62. Photoluminescence reveals an 18-fold enhancement in emission intensity relative to WS<sub>2</sub> on quartz, driven by strong near-field confinement and an increased optical density of states. This approach provides a robust pathway to boost excitonic absorption and emission, advancing integrated optoelectronic platforms based on atomically thin crystals.

Optics LettersVol. 50(24)
Openalex Percentile: Top 31%
2D Materials and Applications
0.52
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Demonstration of Miexciton: enhancement of light–matter interaction in monolayer WS <sub>2</sub> on a Si metasurface — Junichi Takahara, Dingwei Chen · Optics Letters (2025) | TGRS Research Map | TGRS