Engineering spatially separated redox sites in donor–acceptor polymers for enhanced hydrogen peroxide photosynthesis
Herein, two conjugated polymers are constructed, achieving an H<sub>2</sub>O<sub>2</sub> production rate of 6668.3 μmol g<sup>-1</sup> h<sup>-1</sup>. The exceptional performance originates from the synergistic effect of the donor-acceptor (D-A) structure achieving spatial separation of the redox sites, thereby promoting performance. This work provides a novel approach for the structural optimization of photocatalysts.
Authors
- Zhenzi Li (ORCID: https://orcid.org/0000-0002-3106-6622)
- Wei Zhou (ORCID: https://orcid.org/0000-0002-2818-0408)
- Liping Guo (ORCID: https://orcid.org/0000-0003-2065-387X)
- Qing Wang (ORCID: https://orcid.org/0000-0002-2618-5694)
- Xuepeng Wang (ORCID: https://orcid.org/0000-0002-6015-8139)
- Lijun Liao (ORCID: https://orcid.org/0000-0002-9131-785X)
- Wenjiao Wang
Institutions
- Qilu University of Technology (CN)
- Shandong Academy of Sciences (CN)
Publication Details
- Journal
- Chemical Communications
- Published
- 2025-01-01
- DOI
- https://doi.org/10.1039/d5cc04715c
- Primary Topic
- Advanced Photocatalysis Techniques
- Type
- article
- Field-Weighted Citation Impact
- 0.00