Magnetic frustration in the Yb-based triangular lattice compound <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">CuYbSe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>
The Yb-based triangular lattice delafossites $A\mathrm{Yb}{X}_{2}$ ($A=\text{alkali}$ metal, $X=\text{O}$, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of ${\mathrm{CuYbSe}}_{2}$ with a perfect triangular lattice of ${\mathrm{Yb}}^{3+}$ moments. Magnetic susceptibility and heat capacity measurements reveal no evidence of long-range magnetic ordering down to 1.8 K in spite of a significant antiferromagnetic exchange between ${\mathrm{Yb}}^{3+}$ moments, suggesting a frustrated magnetic system. Electrical resistivity measurements indicate insulating behavior, consistent with the localized nature of magnetic moments. Heat capacity reveals that ${\mathrm{CuYbSe}}_{2}$ can be treated as an effective spin $S=1/2$ triangular lattice antiferromagnet below $\ensuremath{\sim}50$ K. Magnetic susceptibility measurements on single crystals reveal weak magnetic anisotropy. These properties position ${\mathrm{CuYbSe}}_{2}$ as another platform for exploring exotic magnetic ground states in triangular lattice systems.
Authors
- Anzar Ali (ORCID: https://orcid.org/0000-0002-6390-7211)
- Masahiko Isobe (ORCID: https://orcid.org/0000-0002-9253-7256)
- Yogesh Singh (ORCID: https://orcid.org/0000-0001-9901-0847)
- Barkha Khattar (ORCID: https://orcid.org/0009-0002-8053-2949)
Institutions
- Indian Institute of Science Education and Research Kolkata (IN)
- Indian Institute of Science Education and Research Mohali (IN)
- Indian Institute of Science Education and Research, Bhopal (IN)
- Max Planck Institute for Solid State Research (DE)
- Indian Institute of Science Education and Research Berhampur (IN)
- Indian Institute of Science Education and Research, Tirupati (IN)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-10-16
- DOI
- https://doi.org/10.1103/5h6v-nm9s
- Primary Topic
- Advanced Condensed Matter Physics
- Type
- article
- Field-Weighted Citation Impact
- 0.00