Magnetic frustration in the Yb-based triangular lattice compound <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">CuYbSe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

The Yb-based triangular lattice delafossites $A\mathrm{Yb}{X}_{2}$ ($A=\text{alkali}$ metal, $X=\text{O}$, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of ${\mathrm{CuYbSe}}_{2}$ with a perfect triangular lattice of ${\mathrm{Yb}}^{3+}$ moments. Magnetic susceptibility and heat capacity measurements reveal no evidence of long-range magnetic ordering down to 1.8 K in spite of a significant antiferromagnetic exchange between ${\mathrm{Yb}}^{3+}$ moments, suggesting a frustrated magnetic system. Electrical resistivity measurements indicate insulating behavior, consistent with the localized nature of magnetic moments. Heat capacity reveals that ${\mathrm{CuYbSe}}_{2}$ can be treated as an effective spin $S=1/2$ triangular lattice antiferromagnet below $\ensuremath{\sim}50$ K. Magnetic susceptibility measurements on single crystals reveal weak magnetic anisotropy. These properties position ${\mathrm{CuYbSe}}_{2}$ as another platform for exploring exotic magnetic ground states in triangular lattice systems.

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Journal
Physical review. B./Physical review. B
Published
2025-10-16
DOI
https://doi.org/10.1103/5h6v-nm9s
Primary Topic
Advanced Condensed Matter Physics
Type
article
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article

Magnetic frustration in the Yb-based triangular lattice compound <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">CuYbSe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

Anzar Ali, Masahiko Isobe, Yogesh Singh, Barkha Khattar
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
article

Magnetic frustration in the Yb-based triangular lattice compound <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">CuYbSe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

Anzar Ali, Masahiko Isobe, Yogesh Singh, Barkha Khattar
article en

Abstract

The Yb-based triangular lattice delafossites $A\mathrm{Yb}{X}_{2}$ ($A=\text{alkali}$ metal, $X=\text{O}$, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of ${\mathrm{CuYbSe}}_{2}$ with a perfect triangular lattice of ${\mathrm{Yb}}^{3+}$ moments. Magnetic susceptibility and heat capacity measurements reveal no evidence of long-range magnetic ordering down to 1.8 K in spite of a significant antiferromagnetic exchange between ${\mathrm{Yb}}^{3+}$ moments, suggesting a frustrated magnetic system. Electrical resistivity measurements indicate insulating behavior, consistent with the localized nature of magnetic moments. Heat capacity reveals that ${\mathrm{CuYbSe}}_{2}$ can be treated as an effective spin $S=1/2$ triangular lattice antiferromagnet below $\ensuremath{\sim}50$ K. Magnetic susceptibility measurements on single crystals reveal weak magnetic anisotropy. These properties position ${\mathrm{CuYbSe}}_{2}$ as another platform for exploring exotic magnetic ground states in triangular lattice systems.

Physical review. B./Physical review. BVol. 112(17)
Indian Institute of Science Education and Research Kolkata (IN), Indian Institute of Science Education and Research Mohali (IN), Indian Institute of Science Education and Research, Bhopal (IN), Max Planck Institute for Solid State Research (DE), Indian Institute of Science Education and Research Berhampur (IN), Indian Institute of Science Education and Research, Tirupati (IN)
Openalex Percentile: Top 80%
Advanced Condensed Matter Physics
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Magnetic frustration in the Yb-based triangular lattice compound <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">CuYbSe</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math> — Anzar Ali, Masahiko Isobe, et al. · Physical review. B./Physical review. B (2025) | TGRS Research Map | TGRS