Absence of magnetic order and magnetic fluctuations in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">RuO</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>
A novel magnetic class blending ferromagnetism and antiferromagnetism, termed altermagnetism, has gained significant attention for its staggered order in coordinate and momentum spaces, time-reversal symmetry-breaking phenomena, and promising applications in spintronics. Ruthenium dioxide (${\mathrm{RuO}}_{2}$) has been considered a candidate material for altermagnetism, yet the presence of magnetic moments on Ru atoms remains a subject of debate. In this study, we systematically investigated the magnetic properties of ${\mathrm{RuO}}_{2}$ powder using nuclear quadrupole resonance (NQR) measurements. The NQR spectra show that there is no internal magnetic field. Furthermore, the temperature independence of spin-lattice relaxation rate, $1/{T}_{1}T$, proves that there are no magnetic fluctuations. Our results unambiguously demonstrate that Ru atoms in ${\mathrm{RuO}}_{2}$ possess neither static magnetic moments nor fluctuating magnetic moments, and thus ${\mathrm{RuO}}_{2}$ does not possess the magnetic characteristics essential for altermagnetism.
Authors
- Xuebo Zhou (ORCID: https://orcid.org/0000-0003-4438-378X)
- Yun‐Ze Long (ORCID: https://orcid.org/0000-0002-4278-4515)
- Jiangpeng Song (ORCID: https://orcid.org/0000-0001-5435-5251)
- Zheng Li (ORCID: https://orcid.org/0000-0001-6946-3474)
- Shilin Zhu (ORCID: https://orcid.org/0009-0005-2928-9113)
- Wei Wu (ORCID: https://orcid.org/0000-0003-4228-2416)
- Jianlin Luo
- Chao Mu (ORCID: https://orcid.org/0000-0001-5751-4342)
Institutions
- Qingdao University (CN)
- Chinese Academy of Sciences (CN)
- FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ)
- Institute of Physics (CN)
- University of Chinese Academy of Sciences (CN)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-10-14
- DOI
- https://doi.org/10.1103/cb99-6thg
- Primary Topic
- Advanced Condensed Matter Physics
- Type
- article
- Field-Weighted Citation Impact
- 0.00