Absence of magnetic order and magnetic fluctuations in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">RuO</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

A novel magnetic class blending ferromagnetism and antiferromagnetism, termed altermagnetism, has gained significant attention for its staggered order in coordinate and momentum spaces, time-reversal symmetry-breaking phenomena, and promising applications in spintronics. Ruthenium dioxide (${\mathrm{RuO}}_{2}$) has been considered a candidate material for altermagnetism, yet the presence of magnetic moments on Ru atoms remains a subject of debate. In this study, we systematically investigated the magnetic properties of ${\mathrm{RuO}}_{2}$ powder using nuclear quadrupole resonance (NQR) measurements. The NQR spectra show that there is no internal magnetic field. Furthermore, the temperature independence of spin-lattice relaxation rate, $1/{T}_{1}T$, proves that there are no magnetic fluctuations. Our results unambiguously demonstrate that Ru atoms in ${\mathrm{RuO}}_{2}$ possess neither static magnetic moments nor fluctuating magnetic moments, and thus ${\mathrm{RuO}}_{2}$ does not possess the magnetic characteristics essential for altermagnetism.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-10-14
DOI
https://doi.org/10.1103/cb99-6thg
Primary Topic
Advanced Condensed Matter Physics
Type
article
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article

Absence of magnetic order and magnetic fluctuations in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">RuO</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

Xuebo Zhou, Yun‐Ze Long, Jiangpeng Song, Zheng Li et al.
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
article

Absence of magnetic order and magnetic fluctuations in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">RuO</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

Xuebo Zhou, Yun‐Ze Long, Jiangpeng Song, Zheng Li, Shilin Zhu, Wei Wu, Jianlin Luo, Chao Mu
article en

Abstract

A novel magnetic class blending ferromagnetism and antiferromagnetism, termed altermagnetism, has gained significant attention for its staggered order in coordinate and momentum spaces, time-reversal symmetry-breaking phenomena, and promising applications in spintronics. Ruthenium dioxide (${\mathrm{RuO}}_{2}$) has been considered a candidate material for altermagnetism, yet the presence of magnetic moments on Ru atoms remains a subject of debate. In this study, we systematically investigated the magnetic properties of ${\mathrm{RuO}}_{2}$ powder using nuclear quadrupole resonance (NQR) measurements. The NQR spectra show that there is no internal magnetic field. Furthermore, the temperature independence of spin-lattice relaxation rate, $1/{T}_{1}T$, proves that there are no magnetic fluctuations. Our results unambiguously demonstrate that Ru atoms in ${\mathrm{RuO}}_{2}$ possess neither static magnetic moments nor fluctuating magnetic moments, and thus ${\mathrm{RuO}}_{2}$ does not possess the magnetic characteristics essential for altermagnetism.

Physical review. B./Physical review. BVol. 112(14)
Qingdao University (CN), Chinese Academy of Sciences (CN), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), Institute of Physics (CN), University of Chinese Academy of Sciences (CN)
Openalex Percentile: Top 80%
Advanced Condensed Matter Physics
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