Comparative analysis of plasmon modes in layered Lindhard metals and strange metals

The enigmatic strange metal remains one of the central unsolved problems of 21st century science. Understanding this phase of matter requires knowledge of the momentum- and energy-resolved dynamic charge susceptibility $\ensuremath{\chi}(q,\ensuremath{\omega})$, especially at finite momentum. Inelastic electron scattering (EELS), performed in either transmission or reflection geometry, is a powerful probe of $\ensuremath{\chi}(q,\ensuremath{\omega})$. For the prototypical strange metal ${\mathrm{Bi}}_{2}{\mathrm{Sr}}_{2}{\mathrm{CaCu}}_{2}{\mathrm{O}}_{8+x}$, transmission- and reflection EELS, and infrared (IR) spectroscopy agree at $q\ensuremath{\sim}0$, all revealing a highly damped plasmon near 1 eV. At larger $q$, however, EELS results show unresolved discrepancies. Since IR data are highly reproducible, it is advantageous to use IR data to calculate what the expected EELS response should be at modest $q$. Building on prior momentum-resolved reflection geometry M-EELS work [Chen et al., Phys. Rev. B 109, 045108 (2024)], we extend this approach to transmission EELS for finite stacks of metallic layers, comparing a ``textbook'' Lindhard metal to a strange metal. In the Lindhard case, the low-$q$ response is dominated by long-lived, standing wave plasmon modes arising from interlayer Coulomb coupling, with in-plane dispersions that resemble the well-known Fetter modes of layered metals. This behavior depends only on the geometry and the long-range nature of the Coulomb interaction and is largely insensitive to layer details. At larger $q$, the response reflects the microscopic properties of individual layers. For the strange metal, calculations based on IR data predict a highly damped plasmon with weak dispersion and no distinct surface mode. While our results match IR and M-EELS at low $q$, they do not reproduce any published EELS spectra at large $q$, highlighting unresolved discrepancies that demand further experimental investigation.

Authors

Institutions

Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-10-15
DOI
https://doi.org/10.1103/39wl-mzly
Primary Topic
Physics of Superconductivity and Magnetism
Type
article
Field-Weighted Citation Impact
0.00
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Comparative analysis of plasmon modes in layered Lindhard metals and strange metals

Dipanjan Chaudhuri, Xuefei Guo, Jordan A. Hachtel, N de Vries et al.
Physical review. B./Physical review. B
Physics of Superconductivity and Magnetism
article

Comparative analysis of plasmon modes in layered Lindhard metals and strange metals

Dipanjan Chaudhuri, Xuefei Guo, Jordan A. Hachtel, N de Vries, Jin Chen, Eric R. Hoglund, Peter Abbamonte
article en

Abstract

The enigmatic strange metal remains one of the central unsolved problems of 21st century science. Understanding this phase of matter requires knowledge of the momentum- and energy-resolved dynamic charge susceptibility $\ensuremath{\chi}(q,\ensuremath{\omega})$, especially at finite momentum. Inelastic electron scattering (EELS), performed in either transmission or reflection geometry, is a powerful probe of $\ensuremath{\chi}(q,\ensuremath{\omega})$. For the prototypical strange metal ${\mathrm{Bi}}_{2}{\mathrm{Sr}}_{2}{\mathrm{CaCu}}_{2}{\mathrm{O}}_{8+x}$, transmission- and reflection EELS, and infrared (IR) spectroscopy agree at $q\ensuremath{\sim}0$, all revealing a highly damped plasmon near 1 eV. At larger $q$, however, EELS results show unresolved discrepancies. Since IR data are highly reproducible, it is advantageous to use IR data to calculate what the expected EELS response should be at modest $q$. Building on prior momentum-resolved reflection geometry M-EELS work [Chen et al., Phys. Rev. B 109, 045108 (2024)], we extend this approach to transmission EELS for finite stacks of metallic layers, comparing a ``textbook'' Lindhard metal to a strange metal. In the Lindhard case, the low-$q$ response is dominated by long-lived, standing wave plasmon modes arising from interlayer Coulomb coupling, with in-plane dispersions that resemble the well-known Fetter modes of layered metals. This behavior depends only on the geometry and the long-range nature of the Coulomb interaction and is largely insensitive to layer details. At larger $q$, the response reflects the microscopic properties of individual layers. For the strange metal, calculations based on IR data predict a highly damped plasmon with weak dispersion and no distinct surface mode. While our results match IR and M-EELS at low $q$, they do not reproduce any published EELS spectra at large $q$, highlighting unresolved discrepancies that demand further experimental investigation.

Physical review. B./Physical review. BVol. 112(16)
Oak Ridge National Laboratory (US), University of Illinois Urbana-Champaign (US)
Openalex Percentile: Top 80%
Physics of Superconductivity and Magnetism
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.