Dynamics of phase-separated interfaces in inhomogeneous and driven mixtures

We derive effective equations of motion governing the dynamics of sharp interfaces in phase-separated binary mixtures driven by spatio-temporal modulations of their material properties. We demonstrate, in particular, that spatial heterogeneities in the surface tension induce an effective capillary force that drives the motion of interfaces, even in the absence of hydrodynamics. Applying our sharp interface model to quantify the dynamics of thermophoretic droplets, we find that their deformation and transport properties are controlled by a combination of bulk and capillary forces, whose relative strength depends on droplet size. Strikingly, we show that small thermophobic droplets - composed of a material with a positive Soret coefficient - can spontaneously migrate towards high-temperature regions as a result of capillary forces.

Authors

Institutions

Publication Details

Journal
Soft Matter
Published
2025-01-01
DOI
https://doi.org/10.1039/d5sm00625b
Citations
1
Primary Topic
Solidification and crystal growth phenomena
Type
article
Field-Weighted Citation Impact
0.52
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Dynamics of phase-separated interfaces in inhomogeneous and driven mixtures

Benoît Mahault, Ramin Golestanian, Jacopo Romano
1 citations
Soft Matter
Solidification and crystal growth phenomena
0.52
article

Dynamics of phase-separated interfaces in inhomogeneous and driven mixtures

Benoît Mahault, Ramin Golestanian, Jacopo Romano
article en
1 citations

Abstract

We derive effective equations of motion governing the dynamics of sharp interfaces in phase-separated binary mixtures driven by spatio-temporal modulations of their material properties. We demonstrate, in particular, that spatial heterogeneities in the surface tension induce an effective capillary force that drives the motion of interfaces, even in the absence of hydrodynamics. Applying our sharp interface model to quantify the dynamics of thermophoretic droplets, we find that their deformation and transport properties are controlled by a combination of bulk and capillary forces, whose relative strength depends on droplet size. Strikingly, we show that small thermophobic droplets - composed of a material with a positive Soret coefficient - can spontaneously migrate towards high-temperature regions as a result of capillary forces.

Soft MatterVol. 21(48)
Scuola Internazionale Superiore di Studi Avanzati (IT), University of Oxford (GB), Max Planck Institute for Dynamics and Self-Organization (DE)
Openalex Percentile: Top 31%
Solidification and crystal growth phenomena
0.52
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.