Flat band driven itinerant magnetism in the Co-pnictides <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">CaCo</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant="normal">As</mml:mi

Flat bands can induce strong electron correlation effects that help stabilize both magnetic and superconducting states. Here, we carry out angle-resolved photoemission spectroscopy and density functional theory calculations to study the electronic structure of the Co-pnictides ${\mathrm{CaCo}}_{2}{\mathrm{As}}_{2}$ and ${\mathrm{LaCo}}_{2}{\mathrm{P}}_{2}$. We find that the ${k}_{z}$ Fermi topology of ferromagnetic ${\mathrm{LaCo}}_{2}{\mathrm{P}}_{2}$ is markedly two-dimensional, while the antiferromagnetic ${\mathrm{CaCo}}_{2}{\mathrm{As}}_{2}$ develops a 3D Fermi surface described by a zigzaglike band dispersion perpendicular to the Co-As plane. Furthermore, the magnetism is driven by the electronic correlations of the flat bands with ${d}_{xy}$ and ${d}_{{z}^{2}}$ orbital character at the Fermi level. Our results link the electronic dimensionality and the magnetic order and emphasize the critical role of the As-As and P-P bond strength along the $c$ direction to understand the electronic band structure and the rich phase diagram of transition metal pnictides.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-09-22
DOI
https://doi.org/10.1103/w9rw-rjdh
Citations
2
Primary Topic
Iron-based superconductors research
Type
article
Field-Weighted Citation Impact
0.85
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article

Flat band driven itinerant magnetism in the Co-pnictides <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">CaCo</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant="normal">As</mml:mi

Dina Carbone, M. Tallarida, Maia G. Vergniory, A. K. Kar et al.
2 citations
Physical review. B./Physical review. B
Iron-based superconductors research
0.85
article

Flat band driven itinerant magnetism in the Co-pnictides <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi mathvariant="normal">CaCo</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant="normal">As</mml:mi

Dina Carbone, M. Tallarida, Maia G. Vergniory, A. K. Kar, E. Vescovo, David Subires, P. Gargiani, Michael Shatruk, Turgut Yilmaz, J. Dai, Vincent Yannello, S. Blanco-Canosa, Victoria M. Li, Mikel García‐Díez, Chaesung Lim
article en
2 citations

Abstract

Flat bands can induce strong electron correlation effects that help stabilize both magnetic and superconducting states. Here, we carry out angle-resolved photoemission spectroscopy and density functional theory calculations to study the electronic structure of the Co-pnictides ${\mathrm{CaCo}}_{2}{\mathrm{As}}_{2}$ and ${\mathrm{LaCo}}_{2}{\mathrm{P}}_{2}$. We find that the ${k}_{z}$ Fermi topology of ferromagnetic ${\mathrm{LaCo}}_{2}{\mathrm{P}}_{2}$ is markedly two-dimensional, while the antiferromagnetic ${\mathrm{CaCo}}_{2}{\mathrm{As}}_{2}$ develops a 3D Fermi surface described by a zigzaglike band dispersion perpendicular to the Co-As plane. Furthermore, the magnetism is driven by the electronic correlations of the flat bands with ${d}_{xy}$ and ${d}_{{z}^{2}}$ orbital character at the Fermi level. Our results link the electronic dimensionality and the magnetic order and emphasize the critical role of the As-As and P-P bond strength along the $c$ direction to understand the electronic band structure and the rich phase diagram of transition metal pnictides.

Physical review. B./Physical review. BVol. 112(16)
Florida State University (US), Ikerbasque (ES), Université de Sherbrooke (CA), University of the Basque Country (ES), Brookhaven National Laboratory (US), ALBA Synchrotron (Spain) (ES), Xiamen University Malaysia (MY), MAX IV Laboratory (SE), Donostia International Physics Center (ES), University of Tampa (US)
Openalex Percentile: Top 24%
Iron-based superconductors research
0.85
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