Magnetoelastic coupling and magnetic anisotropy in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>CoFeO</mml:mi> <mml:mn>6</mml:mn> </mml:msub> </m

The coupling between strain and magnetic order arises due to the modifications in orbital overlap and crystal field symmetry, giving rise to strain-induced magnetic anisotropy. Here, we find an evolution of strain-tuned out-of-plane magnetic anisotropy in thin films of double perovskite ${\mathrm{Sm}}_{2}{\mathrm{CoFeO}}_{6}$, which possesses room-temperature ferromagnetism. Notably, the magnetization of the thin films is enhanced nearly 40 times compared to its bulk value, making a strong case for strain-induced ferromagnetism. The intrinsic magnetic anisotropy constant increases from 3 ${\mathrm{kJ}/\mathrm{m}}^{3}$ to 120 ${\mathrm{kJ}/\mathrm{m}}^{3}$ with the application of tensile strain from 0.7% to 2%. The magnetostriction coefficient is estimated to be as large as $30\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6}$. The strain-induced ferromagnetism in ${\mathrm{Sm}}_{2}{\mathrm{CoFeO}}_{6}$ is well supported with density functional theory calculations. Such magnetoelastic coupling-driven magnetic anisotropy tuning is further discussed in the micromagnetic framework.

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Journal
Physical review. B./Physical review. B
Published
2025-10-03
DOI
https://doi.org/10.1103/dvsj-y8ct
Primary Topic
Multiferroics and related materials
Type
article
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article

Magnetoelastic coupling and magnetic anisotropy in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>CoFeO</mml:mi> <mml:mn>6</mml:mn> </mml:msub> </m

D. Samal, P. S. Anil Kumar, Shwetha G. Bhat, Chanchal Sow et al.
Physical review. B./Physical review. B
Multiferroics and related materials
article

Magnetoelastic coupling and magnetic anisotropy in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>CoFeO</mml:mi> <mml:mn>6</mml:mn> </mml:msub> </m

D. Samal, P. S. Anil Kumar, Shwetha G. Bhat, Chanchal Sow, Digbijaya Palai, Amitava Ghosh, R. J. Choudhary, Wakeel Ahmad
article en

Abstract

The coupling between strain and magnetic order arises due to the modifications in orbital overlap and crystal field symmetry, giving rise to strain-induced magnetic anisotropy. Here, we find an evolution of strain-tuned out-of-plane magnetic anisotropy in thin films of double perovskite ${\mathrm{Sm}}_{2}{\mathrm{CoFeO}}_{6}$, which possesses room-temperature ferromagnetism. Notably, the magnetization of the thin films is enhanced nearly 40 times compared to its bulk value, making a strong case for strain-induced ferromagnetism. The intrinsic magnetic anisotropy constant increases from 3 ${\mathrm{kJ}/\mathrm{m}}^{3}$ to 120 ${\mathrm{kJ}/\mathrm{m}}^{3}$ with the application of tensile strain from 0.7% to 2%. The magnetostriction coefficient is estimated to be as large as $30\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6}$. The strain-induced ferromagnetism in ${\mathrm{Sm}}_{2}{\mathrm{CoFeO}}_{6}$ is well supported with density functional theory calculations. Such magnetoelastic coupling-driven magnetic anisotropy tuning is further discussed in the micromagnetic framework.

Physical review. B./Physical review. BVol. 112(13)
Institute of Physics, Bhubaneshwar (IN), UGC DAE Consortium for Scientific Research (IN), Indian Institute of Science Bangalore (IN), Indian Institute of Technology Kanpur (IN)
Openalex Percentile: Top 78%
Multiferroics and related materials
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