Magnetoelastic coupling and magnetic anisotropy in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Sm</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>CoFeO</mml:mi> <mml:mn>6</mml:mn> </mml:msub> </m
The coupling between strain and magnetic order arises due to the modifications in orbital overlap and crystal field symmetry, giving rise to strain-induced magnetic anisotropy. Here, we find an evolution of strain-tuned out-of-plane magnetic anisotropy in thin films of double perovskite ${\mathrm{Sm}}_{2}{\mathrm{CoFeO}}_{6}$, which possesses room-temperature ferromagnetism. Notably, the magnetization of the thin films is enhanced nearly 40 times compared to its bulk value, making a strong case for strain-induced ferromagnetism. The intrinsic magnetic anisotropy constant increases from 3 ${\mathrm{kJ}/\mathrm{m}}^{3}$ to 120 ${\mathrm{kJ}/\mathrm{m}}^{3}$ with the application of tensile strain from 0.7% to 2%. The magnetostriction coefficient is estimated to be as large as $30\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6}$. The strain-induced ferromagnetism in ${\mathrm{Sm}}_{2}{\mathrm{CoFeO}}_{6}$ is well supported with density functional theory calculations. Such magnetoelastic coupling-driven magnetic anisotropy tuning is further discussed in the micromagnetic framework.
Authors
- D. Samal (ORCID: https://orcid.org/0000-0003-2618-4445)
- P. S. Anil Kumar (ORCID: https://orcid.org/0000-0002-4574-0868)
- Shwetha G. Bhat (ORCID: https://orcid.org/0000-0003-4237-9082)
- Chanchal Sow (ORCID: https://orcid.org/0000-0002-5817-3161)
- Digbijaya Palai (ORCID: https://orcid.org/0009-0005-9700-4511)
- Amitava Ghosh (ORCID: https://orcid.org/0009-0006-4788-161X)
- R. J. Choudhary (ORCID: https://orcid.org/0009-0004-4035-2737)
- Wakeel Ahmad (ORCID: https://orcid.org/0009-0001-0946-9994)
Institutions
- Institute of Physics, Bhubaneshwar (IN)
- UGC DAE Consortium for Scientific Research (IN)
- Indian Institute of Science Bangalore (IN)
- Indian Institute of Technology Kanpur (IN)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-10-03
- DOI
- https://doi.org/10.1103/dvsj-y8ct
- Primary Topic
- Multiferroics and related materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00