Probing Hole-Magnon Dynamics in an Antiferromagnet with Beyond-Nearest-Neighbor Couplings

We study the real-time dynamics of a single hole in a 2D antiferromagnet with long-range couplings. Using an extended <i>t</i>-<i>J</i> model that includes nearest-neighbor (NN) and next-nearest-neighbor (NNN) hopping and superexchange, and the multiple Davydov Ansatz as a numerically accurate variational solver, we track hole-magnon dynamics on an 8 × 8 lattice. We show that even moderate frustrating NNN exchange qualitatively changes the magnetic polaron dynamics: frustration initially promotes transient self-localization but at longer times opens additional propagation channels that increase the root-mean-squared displacement. Our results emphasize that modest beyond-NN interactions can substantially modify magnetic polaron formation and transport, with implications for high-<i>T</i><sub><i>c</i></sub> cuprates and cold-atom quantum simulators.

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Publication Details

Journal
The Journal of Physical Chemistry Letters
Published
2025-10-27
DOI
https://doi.org/10.1021/acs.jpclett.5c03005
Primary Topic
Physics of Superconductivity and Magnetism
Type
article
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article

Probing Hole-Magnon Dynamics in an Antiferromagnet with Beyond-Nearest-Neighbor Couplings

Maxim F. Gelin, Siyuan Luo, Kaijun Shen, Yang Zhao et al.
The Journal of Physical Chemistry Letters
Physics of Superconductivity and Magnetism
article

Probing Hole-Magnon Dynamics in an Antiferromagnet with Beyond-Nearest-Neighbor Couplings

Maxim F. Gelin, Siyuan Luo, Kaijun Shen, Yang Zhao, Kewei Sun
article en

Abstract

We study the real-time dynamics of a single hole in a 2D antiferromagnet with long-range couplings. Using an extended <i>t</i>-<i>J</i> model that includes nearest-neighbor (NN) and next-nearest-neighbor (NNN) hopping and superexchange, and the multiple Davydov Ansatz as a numerically accurate variational solver, we track hole-magnon dynamics on an 8 × 8 lattice. We show that even moderate frustrating NNN exchange qualitatively changes the magnetic polaron dynamics: frustration initially promotes transient self-localization but at longer times opens additional propagation channels that increase the root-mean-squared displacement. Our results emphasize that modest beyond-NN interactions can substantially modify magnetic polaron formation and transport, with implications for high-<i>T</i><sub><i>c</i></sub> cuprates and cold-atom quantum simulators.

The Journal of Physical Chemistry LettersVol. 16(44)
Nanyang Technological University (SG), Hangzhou Dianzi University (CN)
Openalex Percentile: Top 80%
Physics of Superconductivity and Magnetism
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