Enabling Weather-Independent Gas Detection through Deep Learning on Light-Activated Sensors
Light-activated gas sensors offer a low-temperature, low-power approach for detecting target species, and their high-performance capabilities make them ideal for practical applications. The direct integration of Bi-doped In<sub>2</sub>O<sub>3</sub> nanofibers onto micro light-emitting diode (μLED) platforms enables high-performance sensors for simultaneous NO<sub>2</sub> and H<sub>2</sub>O detection. Introducing Bi into In<sub>2</sub>O<sub>3</sub> matrices facilitates the formation of oxygen vacancies and the dissociative adsorption of H<sub>2</sub>O, enhancing the adsorption and reactions with NO<sub>2</sub>. Under blue illumination, this μLED sensor system exhibits high NO<sub>2</sub> sensitivity, with a response value (<i>R</i><sub>g</sub>/<i>R</i><sub>a</sub>) of 264.9 at 1 ppm and 60% relative humidity and response and recovery times of less than 30 s. The use of μLEDs enhances light activation with a high energy transfer efficiency, resulting in outstanding NO<sub>2</sub> sensing characteristics. A convolutional neural network-based algorithm is employed to analyze transient sensing signals, accurately predicting with 99% classification accuracy and 10% regression error for both NO<sub>2</sub> and H<sub>2</sub>O, thereby demonstrating weather-independent sensing. This integration of Bi-doped In<sub>2</sub>O<sub>3</sub> nanofibers, which are specifically activated by blue illumination, μLEDs, and deep learning analytics, enables highly effective real-time environmental monitoring of NO<sub>2</sub> and humidity under environmentally variable outdoor conditions.
Authors
- Jihan Kim (ORCID: https://orcid.org/0000-0002-3844-8789)
- Il‐Doo Kim (ORCID: https://orcid.org/0000-0002-9970-2218)
- Baul Kim (ORCID: https://orcid.org/0000-0002-7983-4336)
- Minhyun Kim (ORCID: https://orcid.org/0000-0003-3679-1775)
- Yunsung Lim (ORCID: https://orcid.org/0000-0002-6327-9286)
- Jaeseok Jeong (ORCID: https://orcid.org/0000-0002-9836-2979)
- Jaewan Ahn (ORCID: https://orcid.org/0000-0002-0136-8427)
- Kichul Lee (ORCID: https://orcid.org/0000-0002-7838-6447)
- Do Y. Kwak (ORCID: https://orcid.org/0000-0002-5743-1501)
- Yong‐Hoon Cho (ORCID: https://orcid.org/0000-0002-7701-8562)
- Inkyu Park (ORCID: https://orcid.org/0000-0001-5761-7739)
- Yeongjae Kwon
- Seyeon Park (ORCID: https://orcid.org/0009-0009-2556-1449)
Institutions
- Korea Advanced Institute of Science and Technology (KR)
- California University of Pennsylvania (US)
- Kootenay Association for Science & Technology (CA)
- University of Pennsylvania (US)
Publication Details
- Journal
- ACS Nano
- Published
- 2025-10-27
- DOI
- https://doi.org/10.1021/acsnano.5c10308
- Citations
- 5
- Primary Topic
- Gas Sensing Nanomaterials and Sensors
- Type
- article
- Field-Weighted Citation Impact
- 3.65