Enabling Weather-Independent Gas Detection through Deep Learning on Light-Activated Sensors

Light-activated gas sensors offer a low-temperature, low-power approach for detecting target species, and their high-performance capabilities make them ideal for practical applications. The direct integration of Bi-doped In<sub>2</sub>O<sub>3</sub> nanofibers onto micro light-emitting diode (μLED) platforms enables high-performance sensors for simultaneous NO<sub>2</sub> and H<sub>2</sub>O detection. Introducing Bi into In<sub>2</sub>O<sub>3</sub> matrices facilitates the formation of oxygen vacancies and the dissociative adsorption of H<sub>2</sub>O, enhancing the adsorption and reactions with NO<sub>2</sub>. Under blue illumination, this μLED sensor system exhibits high NO<sub>2</sub> sensitivity, with a response value (<i>R</i><sub>g</sub>/<i>R</i><sub>a</sub>) of 264.9 at 1 ppm and 60% relative humidity and response and recovery times of less than 30 s. The use of μLEDs enhances light activation with a high energy transfer efficiency, resulting in outstanding NO<sub>2</sub> sensing characteristics. A convolutional neural network-based algorithm is employed to analyze transient sensing signals, accurately predicting with 99% classification accuracy and 10% regression error for both NO<sub>2</sub> and H<sub>2</sub>O, thereby demonstrating weather-independent sensing. This integration of Bi-doped In<sub>2</sub>O<sub>3</sub> nanofibers, which are specifically activated by blue illumination, μLEDs, and deep learning analytics, enables highly effective real-time environmental monitoring of NO<sub>2</sub> and humidity under environmentally variable outdoor conditions.

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Publication Details

Journal
ACS Nano
Published
2025-10-27
DOI
https://doi.org/10.1021/acsnano.5c10308
Citations
5
Primary Topic
Gas Sensing Nanomaterials and Sensors
Type
article
Field-Weighted Citation Impact
3.65
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article

Enabling Weather-Independent Gas Detection through Deep Learning on Light-Activated Sensors

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5 citations
ACS Nano
Gas Sensing Nanomaterials and Sensors
3.65
article

Enabling Weather-Independent Gas Detection through Deep Learning on Light-Activated Sensors

Jihan Kim, Il‐Doo Kim, Baul Kim, Minhyun Kim, Yunsung Lim, Jaeseok Jeong, Jaewan Ahn, Kichul Lee, Do Y. Kwak, Yong‐Hoon Cho, Inkyu Park, Yeongjae Kwon, Seyeon Park
article en
5 citations

Abstract

Light-activated gas sensors offer a low-temperature, low-power approach for detecting target species, and their high-performance capabilities make them ideal for practical applications. The direct integration of Bi-doped In<sub>2</sub>O<sub>3</sub> nanofibers onto micro light-emitting diode (μLED) platforms enables high-performance sensors for simultaneous NO<sub>2</sub> and H<sub>2</sub>O detection. Introducing Bi into In<sub>2</sub>O<sub>3</sub> matrices facilitates the formation of oxygen vacancies and the dissociative adsorption of H<sub>2</sub>O, enhancing the adsorption and reactions with NO<sub>2</sub>. Under blue illumination, this μLED sensor system exhibits high NO<sub>2</sub> sensitivity, with a response value (<i>R</i><sub>g</sub>/<i>R</i><sub>a</sub>) of 264.9 at 1 ppm and 60% relative humidity and response and recovery times of less than 30 s. The use of μLEDs enhances light activation with a high energy transfer efficiency, resulting in outstanding NO<sub>2</sub> sensing characteristics. A convolutional neural network-based algorithm is employed to analyze transient sensing signals, accurately predicting with 99% classification accuracy and 10% regression error for both NO<sub>2</sub> and H<sub>2</sub>O, thereby demonstrating weather-independent sensing. This integration of Bi-doped In<sub>2</sub>O<sub>3</sub> nanofibers, which are specifically activated by blue illumination, μLEDs, and deep learning analytics, enables highly effective real-time environmental monitoring of NO<sub>2</sub> and humidity under environmentally variable outdoor conditions.

ACS NanoVol. 19(44)
Korea Advanced Institute of Science and Technology (KR), California University of Pennsylvania (US), Kootenay Association for Science & Technology (CA), University of Pennsylvania (US)
Openalex Percentile: Top 6%
Gas Sensing Nanomaterials and Sensors
3.65
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