Ultrafast Saddletronics: Current and Charge Control at the M Point

Low-energy valleys in the band structure of 2d materials represent a potential route to the ultrafast writing of information in quantum matter by laser light, with excited charge at the K or K* valleys representing the fundamental states of 1 and 0. Here we demonstrate that a second electronic feature, the saddle point, is endowed with light-wave control over information states. Linearly polarized light is shown to excite 2 of the 3 inequivalent M point saddles in graphene, generating three possible excited configurations, with which of these are realized determined by the polarization vector direction. We show that saddle excitation is highly robust, with "saddle polarized" states created both in the subcycle strong field regime and the multicycle pulse regime. Our findings, applicable to other members of the graphene family and Xenes such as stanene, point toward a rich and ultrafast light-based manipulation of matter based on the saddle point.

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Publication Details

Journal
ACS Nano
Published
2025-10-27
DOI
https://doi.org/10.1021/acsnano.5c02017
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
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article

Ultrafast Saddletronics: Current and Charge Control at the M Point

Deepika Gill, Sam Shallcross, J. K. Dewhurst, S. Sharma et al.
ACS Nano
2D Materials and Applications
article

Ultrafast Saddletronics: Current and Charge Control at the M Point

Deepika Gill, Sam Shallcross, J. K. Dewhurst, S. Sharma, Peter Elliott
article en

Abstract

Low-energy valleys in the band structure of 2d materials represent a potential route to the ultrafast writing of information in quantum matter by laser light, with excited charge at the K or K* valleys representing the fundamental states of 1 and 0. Here we demonstrate that a second electronic feature, the saddle point, is endowed with light-wave control over information states. Linearly polarized light is shown to excite 2 of the 3 inequivalent M point saddles in graphene, generating three possible excited configurations, with which of these are realized determined by the polarization vector direction. We show that saddle excitation is highly robust, with "saddle polarized" states created both in the subcycle strong field regime and the multicycle pulse regime. Our findings, applicable to other members of the graphene family and Xenes such as stanene, point toward a rich and ultrafast light-based manipulation of matter based on the saddle point.

ACS NanoVol. 19(43)
Science and Technology Facilities Council (GB), Max Planck Institute of Microstructure Physics (DE), Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE), Freie Universität Berlin (DE)
Openalex Percentile: Top 76%
2D Materials and Applications
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