Multimagnon and multispinon <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>L</mml:mi> <mml:mn>3</mml:mn> </mml:msub> </mml:math> -edge RIXS spectra of an effective <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"

We investigate the multimagnon and the multispinon ${L}_{3}$-edge resonant inelastic x-ray scattering (RIXS) spectra of a spin-1/2 effective ${\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{J}}_{1}\ensuremath{-}{\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{J}}_{2}\ensuremath{-}{\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{J}}_{3}$ square lattice Heisenberg model in its N\'eel ordered phase. Motivated by the observation of satellite intensity peaks above the single magnon dispersion in the $L$-edge RIXS spectrum, we propose a resonating valence bond (RVB) inspired RIXS mechanism that incorporates the local site ultrashort core-hole lifetime (UCL) expansion. We compute the multimagnon and the multispinon excitations using $O(1/S)$ interacting spin-wave theory and Schwinger boson mean-field theory (SBMFT) formalism, respectively. We treat the x-ray scattering process up to second order in the UCL expansion. Our calculations of two-magnon, bimagnon, and three-magnon RIXS intensities reveal that interacting spin-wave theory fails to fully capture all the quantum correlations in the antiferromagnetic ordered phase. However utilizing the SBMFT framework, with a ground state that incorporates features of both the N\'eel order and fluctuating RVB components, we demonstrate that a RIXS bond-flipping mechanism provides an alternative deeper physical explanation of the satellite intensities. Specifically, we find that the spin-correlation spectra predicted by the fluctuating RVB mechanism aligns with higher-order UCL expansion results. We further show that the satellite intensity above the single-magnon mode can originate both from a one-to-three-magnon hybridization vertex process and from condensed spinons exhibiting Higgs mechanism. These features reflect the interplay of quantum fluctuation, entanglement, and gauge interaction effects of quantum magnetism probed by RIXS.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-10-02
DOI
https://doi.org/10.1103/vc7b-15sf
Primary Topic
Physics of Superconductivity and Magnetism
Type
article
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article

Multimagnon and multispinon <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>L</mml:mi> <mml:mn>3</mml:mn> </mml:msub> </mml:math> -edge RIXS spectra of an effective <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"

Kai-Yuan Qi, Dao‐Xin Yao, Shangjian Jin, Trinanjan Datta
Physical review. B./Physical review. B
Physics of Superconductivity and Magnetism
article

Multimagnon and multispinon <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>L</mml:mi> <mml:mn>3</mml:mn> </mml:msub> </mml:math> -edge RIXS spectra of an effective <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"

Kai-Yuan Qi, Dao‐Xin Yao, Shangjian Jin, Trinanjan Datta
article en

Abstract

We investigate the multimagnon and the multispinon ${L}_{3}$-edge resonant inelastic x-ray scattering (RIXS) spectra of a spin-1/2 effective ${\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{J}}_{1}\ensuremath{-}{\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{J}}_{2}\ensuremath{-}{\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{J}}_{3}$ square lattice Heisenberg model in its N\'eel ordered phase. Motivated by the observation of satellite intensity peaks above the single magnon dispersion in the $L$-edge RIXS spectrum, we propose a resonating valence bond (RVB) inspired RIXS mechanism that incorporates the local site ultrashort core-hole lifetime (UCL) expansion. We compute the multimagnon and the multispinon excitations using $O(1/S)$ interacting spin-wave theory and Schwinger boson mean-field theory (SBMFT) formalism, respectively. We treat the x-ray scattering process up to second order in the UCL expansion. Our calculations of two-magnon, bimagnon, and three-magnon RIXS intensities reveal that interacting spin-wave theory fails to fully capture all the quantum correlations in the antiferromagnetic ordered phase. However utilizing the SBMFT framework, with a ground state that incorporates features of both the N\'eel order and fluctuating RVB components, we demonstrate that a RIXS bond-flipping mechanism provides an alternative deeper physical explanation of the satellite intensities. Specifically, we find that the spin-correlation spectra predicted by the fluctuating RVB mechanism aligns with higher-order UCL expansion results. We further show that the satellite intensity above the single-magnon mode can originate both from a one-to-three-magnon hybridization vertex process and from condensed spinons exhibiting Higgs mechanism. These features reflect the interplay of quantum fluctuation, entanglement, and gauge interaction effects of quantum magnetism probed by RIXS.

Physical review. B./Physical review. BVol. 112(13)
Sun Yat-sen University (CN), Augusta University (US), Augusta University Health (US)
Openalex Percentile: Top 81%
Physics of Superconductivity and Magnetism
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