Electronic structures and Zeeman splitting in GaAs1-xBix nanowires under axial magnetic fields

Combining the effective-mass theory with valence-band anticrossing model, we investigate the electronic structures and Zeeman splitting characteristics of dilute bismuth GaAs nanowires under axial magnetic fields. Calculated results demonstrate that absorption spectra of GaAs<sub>1-<i>x</i></sub> Bi <sub><i>x</i></sub> nanowires exhibit a linear relationship of Zeeman splitting energy with magnetic field regardless of the diameter and Bi composition, due to lifting of degeneracy in both electron and hole states. Importantly, we find that enhanced Zeeman splitting energies and effective <i>g</i> factors of GaAs<sub>1-<i>x</i></sub> Bi <sub><i>x</i></sub> nanowires with larger diameters and lower Bi concentrations can be obtained, which principally arises from splitting energy of the hole states involved in first peaks of <i>σ</i> <sup>+</sup> and <i>σ</i> <sup>-</sup> spectra. Further, normalized magnetic circular dichroism spectra corroborate the Zeeman splitting features observed in the absorption spectra. Our research manifests that GaAs<sub>1-<i>x</i></sub> Bi <sub><i>x</i></sub> nanowires exhibit promising potential for quantum information processing applications because of their large and tunable effective <i>g</i> factors.

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Publication Details

Journal
iScience
Published
2025-10-25
DOI
https://doi.org/10.1016/j.isci.2025.113829
Primary Topic
Semiconductor Quantum Structures and Devices
Type
article
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article

Electronic structures and Zeeman splitting in GaAs1-xBix nanowires under axial magnetic fields

Xin Li, Wen Xiong, Jiarui Zhang, Zhiying Hu
iScience
Semiconductor Quantum Structures and Devices
article

Electronic structures and Zeeman splitting in GaAs1-xBix nanowires under axial magnetic fields

Xin Li, Wen Xiong, Jiarui Zhang, Zhiying Hu
article en

Abstract

Combining the effective-mass theory with valence-band anticrossing model, we investigate the electronic structures and Zeeman splitting characteristics of dilute bismuth GaAs nanowires under axial magnetic fields. Calculated results demonstrate that absorption spectra of GaAs<sub>1-<i>x</i></sub> Bi <sub><i>x</i></sub> nanowires exhibit a linear relationship of Zeeman splitting energy with magnetic field regardless of the diameter and Bi composition, due to lifting of degeneracy in both electron and hole states. Importantly, we find that enhanced Zeeman splitting energies and effective <i>g</i> factors of GaAs<sub>1-<i>x</i></sub> Bi <sub><i>x</i></sub> nanowires with larger diameters and lower Bi concentrations can be obtained, which principally arises from splitting energy of the hole states involved in first peaks of <i>σ</i> <sup>+</sup> and <i>σ</i> <sup>-</sup> spectra. Further, normalized magnetic circular dichroism spectra corroborate the Zeeman splitting features observed in the absorption spectra. Our research manifests that GaAs<sub>1-<i>x</i></sub> Bi <sub><i>x</i></sub> nanowires exhibit promising potential for quantum information processing applications because of their large and tunable effective <i>g</i> factors.

iScienceVol. 28(11)
Chongqing University of Posts and Telecommunications (CN), Chongqing Institute of Green and Intelligent Technology (CN), University of Chinese Academy of Sciences (CN)
Openalex Percentile: Top 75%
Semiconductor Quantum Structures and Devices
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