Quantum path control in high-order harmonic generation via squeezed light

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths (short and long quantum paths) contributing to harmonic emission. Here we demonstrate that these quantum paths in HHG can be selectively controlled using squeezed light, a form of nonclassical light. Our results indicate that the long (short) quantum path of HHG will be dramatically suppressed in the phase (amplitude)-squeezed fields. The time-frequency analysis reveals that this quantum path control stems from the quantum fluctuations in the squeezed light, which modify the phase matching of harmonic emission from different quantum states of the squeezed light. Such a quantum path selection can be achieved for the whole harmonic plateau, which has great potential to generate ultrashort isolated attosecond pulses with duration less than one atomic unit of time.

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Publication Details

Journal
Physical review. A/Physical review, A
Published
2025-09-22
DOI
https://doi.org/10.1103/hph3-kzb2
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
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article

Quantum path control in high-order harmonic generation via squeezed light

Pengfei Lan, Qing Liao, Chunhui Yang, Xinyi Cui et al.
Physical review. A/Physical review, A
Laser-Matter Interactions and Applications
article

Quantum path control in high-order harmonic generation via squeezed light

Pengfei Lan, Qing Liao, Chunhui Yang, Xinyi Cui, Feng Wang, Peixiang Lu, Lixin He, Rui‐Bo Jin, Tianxin Ou
article en

Abstract

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths (short and long quantum paths) contributing to harmonic emission. Here we demonstrate that these quantum paths in HHG can be selectively controlled using squeezed light, a form of nonclassical light. Our results indicate that the long (short) quantum path of HHG will be dramatically suppressed in the phase (amplitude)-squeezed fields. The time-frequency analysis reveals that this quantum path control stems from the quantum fluctuations in the squeezed light, which modify the phase matching of harmonic emission from different quantum states of the squeezed light. Such a quantum path selection can be achieved for the whole harmonic plateau, which has great potential to generate ultrashort isolated attosecond pulses with duration less than one atomic unit of time.

Physical review. A/Physical review, AVol. 112(4)
Wuhan National Laboratory for Optoelectronics (CN), Huazhong University of Science and Technology (CN), Wuhan Institute of Technology (CN)
Openalex Percentile: Top 75%
Laser-Matter Interactions and Applications
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Quantum path control in high-order harmonic generation via squeezed light — Pengfei Lan, Qing Liao, et al. · Physical review. A/Physical review, A (2025) | TGRS Research Map | TGRS