Confinement-driven renormalization of magnon and phonon spectra in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Fe</mml:mi> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant="normal">O</mml:mi> <

The authors reveal here how finite-size confinement reshapes spin and lattice excitations in Fe${}_{3}$O${}_{4}$ nanoparticles using time-of-flight neutron spectroscopy and numerical simulations. Confinement induces surface strain that softens and broadens optical phonons, while surface exchange disorder suppresses acoustic magnon velocities. Molecular dynamics captures size-dependent phonon renormalization, and a reduced-exchange spin-wave model reproduces the magnon behavior. These results establish confinement as a powerful route to tailor spin dynamics and thermal transport in magnetic nanomaterials.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-10-07
DOI
https://doi.org/10.1103/15zz-8g6x
Citations
1
Primary Topic
Multiferroics and related materials
Type
article
Field-Weighted Citation Impact
0.43
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article

Confinement-driven renormalization of magnon and phonon spectra in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Fe</mml:mi> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant="normal">O</mml:mi> <

Dehong Yu, Zhenxiang Cheng, Pablo Galaviz, K. C. Rule et al.
1 citations
Physical review. B./Physical review. B
Multiferroics and related materials
0.43
article

Confinement-driven renormalization of magnon and phonon spectra in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Fe</mml:mi> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant="normal">O</mml:mi> <

Dehong Yu, Zhenxiang Cheng, Pablo Galaviz, K. C. Rule, David Cortie, Kyle A. Portwin
article en
1 citations

Abstract

The authors reveal here how finite-size confinement reshapes spin and lattice excitations in Fe${}_{3}$O${}_{4}$ nanoparticles using time-of-flight neutron spectroscopy and numerical simulations. Confinement induces surface strain that softens and broadens optical phonons, while surface exchange disorder suppresses acoustic magnon velocities. Molecular dynamics captures size-dependent phonon renormalization, and a reduced-exchange spin-wave model reproduces the magnon behavior. These results establish confinement as a powerful route to tailor spin dynamics and thermal transport in magnetic nanomaterials.

Physical review. B./Physical review. BVol. 112(14)
Australian Nuclear Science and Technology Organisation (AU), University of Wollongong (AU)
Openalex Percentile: Top 35%
Multiferroics and related materials
0.43
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Confinement-driven renormalization of magnon and phonon spectra in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Fe</mml:mi> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant="normal">O</mml:mi> < — Dehong Yu, Zhenxiang Cheng, et al. · Physical review. B./Physical review. B (2025) | TGRS Research Map | TGRS