Low-lying electronic structure of the rare earth based topological nodal line semimetal candidate DySbTe
Lanthanide ($Ln$) based $Ln\mathrm{SbTe}$ materials have garnered significant attention due to the rich interplay of long-range magnetic ordering and topological properties, driven by unique crystalline symmetry, $4f$ electron interactions, and pronounced spin-orbit coupling (SOC) effects. DySbTe, as a heavier lanthanide based member of the $Ln\mathrm{SbTe}$ family, stands out with its SOC and larger on-site interactions on its $4f$ electrons, which arise due to the heavier Dy element. Here, we present a comprehensive study on the low-temperature bulk physical properties and the electronic structure of DySbTe using magnetic susceptibility, heat capacity, and electrical resistivity measurements, along with high-resolution angle-resolved photoemission spectroscopy (ARPES), scanning tunneling microscopy and spectroscopy (STM/S), and density functional theory calculations. Our thermodynamic measurements revealed an antiferromagnetic ordering below ${T}_{\mathrm{N}}=7.45$ K and a subsequent magnetic phase transition at ${T}_{\mathrm{N}1}=7.15$ K. Our transport studies indicate a semimetallic behavior with unusual feature in the ordered state. Our ARPES measurements revealed a diamond-shaped Fermi pocket centered at the $\overline{\mathrm{\ensuremath{\Gamma}}}$ point, with band features that evolve distinctly across various binding energies. STM/S results indicate a minimum in the density of states at around 100 meV below the Fermi level, and ARPES measurements reveal a significant gap present around the $\overline{\mathrm{X}}$ point, differentiating DySbTe from other $Ln\mathrm{SbTe}$ compounds. These findings enhance our understanding of the SOC effects on the electronic structure and topological properties in the $Ln\mathrm{SbTe}$ family, highlighting DySbTe as a promising candidate for exploring the interplay between topology and magnetism.
Authors
- Douglas R. James (ORCID: https://orcid.org/0009-0003-6007-9400)
- D. Kaczorowski (ORCID: https://orcid.org/0000-0002-8513-7422)
- Andrzej Ptok (ORCID: https://orcid.org/0000-0002-5566-2656)
- Florie Mesple (ORCID: https://orcid.org/0009-0007-0239-1534)
- Grzegorz Chajewski (ORCID: https://orcid.org/0000-0001-7700-9685)
- Matthew Yankowitz (ORCID: https://orcid.org/0000-0002-5637-9203)
- Tetiana Romanova (ORCID: https://orcid.org/0000-0002-0704-188X)
- Madhab Neupane (ORCID: https://orcid.org/0000-0002-8288-8474)
- Nathan Valadez (ORCID: https://orcid.org/0009-0002-3452-3822)
- Iftakhar Bin Elius (ORCID: https://orcid.org/0000-0002-1056-3320)
- Ellis Thompson (ORCID: https://orcid.org/0009-0002-8499-2360)
- Keng Tou Chu (ORCID: https://orcid.org/0009-0006-1627-2643)
- Peter Radanovich
- Sami Elgalal (ORCID: https://orcid.org/0009-0008-9032-7985)
Institutions
- University of Central Florida (US)
- University of Washington (US)
- Polish Academy of Sciences (PL)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-10-21
- DOI
- https://doi.org/10.1103/s56l-5563
- Citations
- 3
- Primary Topic
- Topological Materials and Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 3.74