Low-lying electronic structure of the rare earth based topological nodal line semimetal candidate DySbTe

Lanthanide ($Ln$) based $Ln\mathrm{SbTe}$ materials have garnered significant attention due to the rich interplay of long-range magnetic ordering and topological properties, driven by unique crystalline symmetry, $4f$ electron interactions, and pronounced spin-orbit coupling (SOC) effects. DySbTe, as a heavier lanthanide based member of the $Ln\mathrm{SbTe}$ family, stands out with its SOC and larger on-site interactions on its $4f$ electrons, which arise due to the heavier Dy element. Here, we present a comprehensive study on the low-temperature bulk physical properties and the electronic structure of DySbTe using magnetic susceptibility, heat capacity, and electrical resistivity measurements, along with high-resolution angle-resolved photoemission spectroscopy (ARPES), scanning tunneling microscopy and spectroscopy (STM/S), and density functional theory calculations. Our thermodynamic measurements revealed an antiferromagnetic ordering below ${T}_{\mathrm{N}}=7.45$ K and a subsequent magnetic phase transition at ${T}_{\mathrm{N}1}=7.15$ K. Our transport studies indicate a semimetallic behavior with unusual feature in the ordered state. Our ARPES measurements revealed a diamond-shaped Fermi pocket centered at the $\overline{\mathrm{\ensuremath{\Gamma}}}$ point, with band features that evolve distinctly across various binding energies. STM/S results indicate a minimum in the density of states at around 100 meV below the Fermi level, and ARPES measurements reveal a significant gap present around the $\overline{\mathrm{X}}$ point, differentiating DySbTe from other $Ln\mathrm{SbTe}$ compounds. These findings enhance our understanding of the SOC effects on the electronic structure and topological properties in the $Ln\mathrm{SbTe}$ family, highlighting DySbTe as a promising candidate for exploring the interplay between topology and magnetism.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-10-21
DOI
https://doi.org/10.1103/s56l-5563
Citations
3
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
3.74
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article

Low-lying electronic structure of the rare earth based topological nodal line semimetal candidate DySbTe

Douglas R. James, D. Kaczorowski, Andrzej Ptok, Florie Mesple et al.
3 citations
Physical review. B./Physical review. B
Topological Materials and Phenomena
3.74
article

Low-lying electronic structure of the rare earth based topological nodal line semimetal candidate DySbTe

Douglas R. James, D. Kaczorowski, Andrzej Ptok, Florie Mesple, Grzegorz Chajewski, Matthew Yankowitz, Tetiana Romanova, Madhab Neupane, Nathan Valadez, Iftakhar Bin Elius, Ellis Thompson, Keng Tou Chu, Peter Radanovich, Sami Elgalal
article en
3 citations

Abstract

Lanthanide ($Ln$) based $Ln\mathrm{SbTe}$ materials have garnered significant attention due to the rich interplay of long-range magnetic ordering and topological properties, driven by unique crystalline symmetry, $4f$ electron interactions, and pronounced spin-orbit coupling (SOC) effects. DySbTe, as a heavier lanthanide based member of the $Ln\mathrm{SbTe}$ family, stands out with its SOC and larger on-site interactions on its $4f$ electrons, which arise due to the heavier Dy element. Here, we present a comprehensive study on the low-temperature bulk physical properties and the electronic structure of DySbTe using magnetic susceptibility, heat capacity, and electrical resistivity measurements, along with high-resolution angle-resolved photoemission spectroscopy (ARPES), scanning tunneling microscopy and spectroscopy (STM/S), and density functional theory calculations. Our thermodynamic measurements revealed an antiferromagnetic ordering below ${T}_{\mathrm{N}}=7.45$ K and a subsequent magnetic phase transition at ${T}_{\mathrm{N}1}=7.15$ K. Our transport studies indicate a semimetallic behavior with unusual feature in the ordered state. Our ARPES measurements revealed a diamond-shaped Fermi pocket centered at the $\overline{\mathrm{\ensuremath{\Gamma}}}$ point, with band features that evolve distinctly across various binding energies. STM/S results indicate a minimum in the density of states at around 100 meV below the Fermi level, and ARPES measurements reveal a significant gap present around the $\overline{\mathrm{X}}$ point, differentiating DySbTe from other $Ln\mathrm{SbTe}$ compounds. These findings enhance our understanding of the SOC effects on the electronic structure and topological properties in the $Ln\mathrm{SbTe}$ family, highlighting DySbTe as a promising candidate for exploring the interplay between topology and magnetism.

Physical review. B./Physical review. BVol. 112(15)
University of Central Florida (US), University of Washington (US), Polish Academy of Sciences (PL)
Openalex Percentile: Top 6%
Topological Materials and Phenomena
3.74
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