Embedding monolayers of 2D materials in directly sputtered monolithic cavities for strong light-matter coupling

We present a monolithic planar Fabry–Pérot microcavity integrating a monolayer of WS 2 using fully sputtered SiO 2 /TiO 2 distributed Bragg reflectors (DBRs). Direct deposition of the top DBR is made possible by protecting the transition metal dichalcogenide monolayer with a thin hexagonal boron nitride (hBN) layer, preserving its optical integrity throughout the fabrication process. The resulting structure supports strong exciton–photon coupling, confirmed by a clear Rabi splitting of (36 ± 4) meV observed in angle-resolved photoluminescence (PL) measurements. This fabrication route avoids complex mechanical assembly or high-temperature processing, offering a robust and scalable alternative for realizing solid-state exciton-polariton systems while allowing precise control of the DBR layer thickness. Our approach simplifies access to monolithic TMDC microcavities, potentially enabling broader experimental exploration of polaritonic and nonlinear optics phenomena.

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Publication Details

Journal
Optical Materials Express
Published
2025-10-21
DOI
https://doi.org/10.1364/ome.576174
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
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article

Embedding monolayers of 2D materials in directly sputtered monolithic cavities for strong light-matter coupling

M. Kamp, Takashi Taniguchi, Kenji Watanabe, Sven Höfling et al.
Optical Materials Express
Strong Light-Matter Interactions
article

Embedding monolayers of 2D materials in directly sputtered monolithic cavities for strong light-matter coupling

M. Kamp, Takashi Taniguchi, Kenji Watanabe, Sven Höfling, Ankur Arora, Simon Betzold, Subhamoy Sahoo, Monika Emmerling, Atanu Patra, Mathias Federolf
article en

Abstract

We present a monolithic planar Fabry–Pérot microcavity integrating a monolayer of WS 2 using fully sputtered SiO 2 /TiO 2 distributed Bragg reflectors (DBRs). Direct deposition of the top DBR is made possible by protecting the transition metal dichalcogenide monolayer with a thin hexagonal boron nitride (hBN) layer, preserving its optical integrity throughout the fabrication process. The resulting structure supports strong exciton–photon coupling, confirmed by a clear Rabi splitting of (36 ± 4) meV observed in angle-resolved photoluminescence (PL) measurements. This fabrication route avoids complex mechanical assembly or high-temperature processing, offering a robust and scalable alternative for realizing solid-state exciton-polariton systems while allowing precise control of the DBR layer thickness. Our approach simplifies access to monolithic TMDC microcavities, potentially enabling broader experimental exploration of polaritonic and nonlinear optics phenomena.

Optical Materials ExpressVol. 16(1)
National Institute for Materials Science (JP)
Openalex Percentile: Top 76%
Strong Light-Matter Interactions
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Embedding monolayers of 2D materials in directly sputtered monolithic cavities for strong light-matter coupling — M. Kamp, Takashi Taniguchi, et al. · Optical Materials Express (2025) | TGRS Research Map | TGRS