Embedding monolayers of 2D materials in directly sputtered monolithic cavities for strong light-matter coupling
We present a monolithic planar Fabry–Pérot microcavity integrating a monolayer of WS 2 using fully sputtered SiO 2 /TiO 2 distributed Bragg reflectors (DBRs). Direct deposition of the top DBR is made possible by protecting the transition metal dichalcogenide monolayer with a thin hexagonal boron nitride (hBN) layer, preserving its optical integrity throughout the fabrication process. The resulting structure supports strong exciton–photon coupling, confirmed by a clear Rabi splitting of (36 ± 4) meV observed in angle-resolved photoluminescence (PL) measurements. This fabrication route avoids complex mechanical assembly or high-temperature processing, offering a robust and scalable alternative for realizing solid-state exciton-polariton systems while allowing precise control of the DBR layer thickness. Our approach simplifies access to monolithic TMDC microcavities, potentially enabling broader experimental exploration of polaritonic and nonlinear optics phenomena.
Authors
- M. Kamp (ORCID: https://orcid.org/0000-0002-7219-2297)
- Takashi Taniguchi (ORCID: https://orcid.org/0000-0002-1467-3105)
- Kenji Watanabe (ORCID: https://orcid.org/0000-0003-3701-8119)
- Sven Höfling (ORCID: https://orcid.org/0000-0003-0034-4682)
- Ankur Arora (ORCID: https://orcid.org/0000-0003-4350-5773)
- Simon Betzold (ORCID: https://orcid.org/0000-0001-9217-1832)
- Subhamoy Sahoo (ORCID: https://orcid.org/0000-0001-5199-2087)
- Monika Emmerling (ORCID: https://orcid.org/0000-0002-4387-0394)
- Atanu Patra (ORCID: https://orcid.org/0000-0002-8151-7997)
- Mathias Federolf
Institutions
- National Institute for Materials Science (JP)
Publication Details
- Journal
- Optical Materials Express
- Published
- 2025-10-21
- DOI
- https://doi.org/10.1364/ome.576174
- Primary Topic
- Strong Light-Matter Interactions
- Type
- article
- Field-Weighted Citation Impact
- 0.00