High-Performance Polarization-Sensitive Photodetector Based on ReS <sub>2</sub> /MoWSe <sub>2</sub> van der Waals Heterostructure
Anisotropic two-dimensional (2D) materials offer a compelling platform for polarized light detection owing to their intrinsic polarization-sensitive optoelectronic responses. However, devices based on single materials often suffer from limited responsivity, narrow spectral coverage, and elevated noise levels. Here we report a high-performance, polarization-sensitive photodetector based on a van der Waals heterostructure composed of anisotropic ReS<sub>2</sub> and a ternary MoWSe<sub>2</sub> alloy. This design couples the polarization-dependent optical response of ReS<sub>2</sub> with the low-defect and highly efficient absorption of MoWSe<sub>2</sub>, achieving a markedly high detectivity of 3.78 × 10<sup>14</sup> Jones and a noticeable polarization ratio of 11.3 under zero or small negative bias. The built-in electric field of the junction effectively suppresses dark current and separates photogenerated carriers rapidly, making the device capable of broadband detection from the visible (405 nm) to near-infrared (1064 nm) spectrum. Under forward bias, the device transitions to a photoconductive regime, achieving a responsivity of 23.22 A/W. These findings highlight the potential of ReS<sub>2</sub>/MoWSe<sub>2</sub> heterostructures as a versatile and scalable platform for broadband, low-noise, and polarization-resolved photodetection, offering a scalable route toward advanced optoelectronic technologies.
Authors
- Zongwen Liu
- Yanping Liu (ORCID: https://orcid.org/0000-0003-2990-3783)
- Shikun Hou (ORCID: https://orcid.org/0000-0003-0139-9730)
- Zhili He (ORCID: https://orcid.org/0000-0001-8225-7333)
- Ding Li (ORCID: https://orcid.org/0000-0001-7286-8907)
- Jun He
- Jian-Tao Wang (ORCID: https://orcid.org/0000-0002-0786-1212)
- Xing Xie (ORCID: https://orcid.org/0000-0002-1636-4816)
- Shaofei Li (ORCID: https://orcid.org/0000-0003-4390-5777)
Institutions
- The University of Sydney (AU)
- Central South University (CN)
- Chinese Academy of Sciences (CN)
- City University of Hong Kong, Shenzhen Research Institute (CN)
- Songshan Lake Materials Laboratory (CN)
- FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ)
- Institute of Physics (CN)
- University of Chinese Academy of Sciences (CN)
Publication Details
- Journal
- ACS Applied Materials & Interfaces
- Published
- 2025-10-21
- DOI
- https://doi.org/10.1021/acsami.5c16945
- Primary Topic
- 2D Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00