High-Performance Polarization-Sensitive Photodetector Based on ReS <sub>2</sub> /MoWSe <sub>2</sub> van der Waals Heterostructure

Anisotropic two-dimensional (2D) materials offer a compelling platform for polarized light detection owing to their intrinsic polarization-sensitive optoelectronic responses. However, devices based on single materials often suffer from limited responsivity, narrow spectral coverage, and elevated noise levels. Here we report a high-performance, polarization-sensitive photodetector based on a van der Waals heterostructure composed of anisotropic ReS<sub>2</sub> and a ternary MoWSe<sub>2</sub> alloy. This design couples the polarization-dependent optical response of ReS<sub>2</sub> with the low-defect and highly efficient absorption of MoWSe<sub>2</sub>, achieving a markedly high detectivity of 3.78 × 10<sup>14</sup> Jones and a noticeable polarization ratio of 11.3 under zero or small negative bias. The built-in electric field of the junction effectively suppresses dark current and separates photogenerated carriers rapidly, making the device capable of broadband detection from the visible (405 nm) to near-infrared (1064 nm) spectrum. Under forward bias, the device transitions to a photoconductive regime, achieving a responsivity of 23.22 A/W. These findings highlight the potential of ReS<sub>2</sub>/MoWSe<sub>2</sub> heterostructures as a versatile and scalable platform for broadband, low-noise, and polarization-resolved photodetection, offering a scalable route toward advanced optoelectronic technologies.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2025-10-21
DOI
https://doi.org/10.1021/acsami.5c16945
Primary Topic
2D Materials and Applications
Type
article
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article

High-Performance Polarization-Sensitive Photodetector Based on ReS 2 /MoWSe 2 van der Waals Heterostructure

Zongwen Liu, Yanping Liu, Shikun Hou, Zhili He et al.
ACS Applied Materials & Interfaces
2D Materials and Applications
article

High-Performance Polarization-Sensitive Photodetector Based on ReS 2 /MoWSe 2 van der Waals Heterostructure

Zongwen Liu, Yanping Liu, Shikun Hou, Zhili He, Ding Li, Jun He, Jian-Tao Wang, Xing Xie, Shaofei Li
article en

Abstract

Anisotropic two-dimensional (2D) materials offer a compelling platform for polarized light detection owing to their intrinsic polarization-sensitive optoelectronic responses. However, devices based on single materials often suffer from limited responsivity, narrow spectral coverage, and elevated noise levels. Here we report a high-performance, polarization-sensitive photodetector based on a van der Waals heterostructure composed of anisotropic ReS<sub>2</sub> and a ternary MoWSe<sub>2</sub> alloy. This design couples the polarization-dependent optical response of ReS<sub>2</sub> with the low-defect and highly efficient absorption of MoWSe<sub>2</sub>, achieving a markedly high detectivity of 3.78 × 10<sup>14</sup> Jones and a noticeable polarization ratio of 11.3 under zero or small negative bias. The built-in electric field of the junction effectively suppresses dark current and separates photogenerated carriers rapidly, making the device capable of broadband detection from the visible (405 nm) to near-infrared (1064 nm) spectrum. Under forward bias, the device transitions to a photoconductive regime, achieving a responsivity of 23.22 A/W. These findings highlight the potential of ReS<sub>2</sub>/MoWSe<sub>2</sub> heterostructures as a versatile and scalable platform for broadband, low-noise, and polarization-resolved photodetection, offering a scalable route toward advanced optoelectronic technologies.

ACS Applied Materials & InterfacesVol. 17(43)
The University of Sydney (AU), Central South University (CN), Chinese Academy of Sciences (CN), City University of Hong Kong, Shenzhen Research Institute (CN), Songshan Lake Materials Laboratory (CN), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), Institute of Physics (CN), University of Chinese Academy of Sciences (CN)
Openalex Percentile: Top 76%
2D Materials and Applications
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